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@ARTICLE{Akola:21034,
author = {Akola, J. and Jones, R. O.},
title = {{S}tructure and dynamics in amorphous tellurium and {T}en
clusters: {A} density functional study},
journal = {Physical review / B},
volume = {85},
number = {13},
issn = {1098-0121},
address = {College Park, Md.},
publisher = {APS},
reportid = {PreJuSER-21034},
pages = {134103},
year = {2012},
note = {The calculations were performed on IBM Blue Gene/P (Jugene)
and Intel Xeon computers in the FZ Julich with grants from
the FZJ and the John von Neumann Institute for Computing
(NIC). We thank S. Kohara for computing the ring
distributions [Fig. 12(a)], J. Heinen and co-workers,
particularly I. Heimbach and F. Rhiem, for developing an
efficient program for cavity analysis, and J. C. Mauro for
providing original data from Ref. 22 [Fig. 7(a)]. J.A.
thanks the Academy of Finland for financial support.},
abstract = {Density functional/molecular dynamics simulations have been
performed on amorphous tellurium (a melt-quenched sample of
343 atoms at 300 K) and on Te clusters with up to 16 atoms.
The former extend our calculations on liquid Te at 560, 625,
722, and 970 K [Phys. Rev. B 81, 094202 (2010)]. We discuss
trends in structures (including those of other group-16
elements), electronic densities of states, and vibration
frequencies. Chain structures are common in S and Se, but
the chains in amorphous Te are short, and branching sites
with threefold-coordinated atoms are common. The energy
difference between two- and threefold local coordination
depends sensitively on the exchange-correlation functional
used. Cavities are characteristic of amorphous Te $(37\%$ of
total volume), but are absent in crystalline (trigonal) Te.},
keywords = {J (WoSType)},
cin = {IAS-1 / PGI-1},
ddc = {530},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106},
pnm = {Grundlagen für zukünftige Informationstechnologien},
pid = {G:(DE-Juel1)FUEK412},
shelfmark = {Physics, Condensed Matter},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000302605400001},
doi = {10.1103/PhysRevB.85.134103},
url = {https://juser.fz-juelich.de/record/21034},
}