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000021323 084__ $$2WoS$$aPhysics, Atomic, Molecular & Chemical
000021323 1001_ $$0P:(DE-Juel1)VDB88605$$aYang, M.$$b0$$uFZJ
000021323 245__ $$aDrift velocity in non-isothermal inhomogeneous systems
000021323 260__ $$aMelville, NY$$bAmerican Institute of Physics$$c2012
000021323 300__ $$a204508
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000021323 440_0 $$03145$$aJournal of Chemical Physics$$v136$$x0021-9606$$y204508
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000021323 520__ $$aDrift velocity and driving force are not directly proportional in the case of inhomogeneous suspensions, where a space dependent mobility induces an additional contribution to the drift velocity. Similarly, particle flux and drift velocity are related not only by the gradient of density but also by an additional contribution given by the gradient of the self-diffusion coefficient. We provide quantitative support to this scenario in a non-equilibrium system by means of computer simulations with a temperature gradient. Moreover, our simulation results demonstrate that the temperature gradient-induced mass transport coefficient, namely thermal diffusion coefficient, is not directly proportional to the drift velocity so that the well-accepted relation of proportionality is just an approximation.
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000021323 650_2 $$2MeSH$$aAlgorithms
000021323 650_2 $$2MeSH$$aComputer Simulation
000021323 650_2 $$2MeSH$$aDiffusion
000021323 650_2 $$2MeSH$$aModels, Chemical
000021323 650_2 $$2MeSH$$aSuspensions
000021323 650_2 $$2MeSH$$aThermodynamics
000021323 650_7 $$00$$2NLM Chemicals$$aSuspensions
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000021323 7001_ $$0P:(DE-Juel1)130920$$aRipoll, M.$$b1$$uFZJ
000021323 773__ $$0PERI:(DE-600)1473050-9$$a10.1063/1.4723685$$gVol. 136$$p204508$$q136$$tThe @journal of chemical physics$$v136$$x0021-9606$$y2012
000021323 8567_ $$uhttp://dx.doi.org/10.1063/1.4723685
000021323 8564_ $$uhttps://juser.fz-juelich.de/record/21323/files/FZJ-21323.pdf$$yPublished under German "Allianz" Licensing conditions on 2012-05-31. Available in OpenAccess from 2012-05-31$$zPublished final document.
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