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005     20240610121023.0
024 7 _ |a pmid:22667572
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024 7 _ |a 10.1063/1.4723685
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037 _ _ |a PreJuSER-21323
041 _ _ |a eng
082 _ _ |a 540
084 _ _ |2 WoS
|a Physics, Atomic, Molecular & Chemical
100 1 _ |a Yang, M.
|b 0
|u FZJ
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245 _ _ |a Drift velocity in non-isothermal inhomogeneous systems
260 _ _ |a Melville, NY
|b American Institute of Physics
|c 2012
300 _ _ |a 204508
336 7 _ |a Journal Article
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336 7 _ |a article
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440 _ 0 |a Journal of Chemical Physics
|x 0021-9606
|0 3145
|y 204508
|v 136
500 _ _ |a Record converted from VDB: 12.11.2012
520 _ _ |a Drift velocity and driving force are not directly proportional in the case of inhomogeneous suspensions, where a space dependent mobility induces an additional contribution to the drift velocity. Similarly, particle flux and drift velocity are related not only by the gradient of density but also by an additional contribution given by the gradient of the self-diffusion coefficient. We provide quantitative support to this scenario in a non-equilibrium system by means of computer simulations with a temperature gradient. Moreover, our simulation results demonstrate that the temperature gradient-induced mass transport coefficient, namely thermal diffusion coefficient, is not directly proportional to the drift velocity so that the well-accepted relation of proportionality is just an approximation.
536 _ _ |a BioSoft: Makromolekulare Systeme und biologische Informationsverarbeitung
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588 _ _ |a Dataset connected to Web of Science, Pubmed
650 _ 2 |2 MeSH
|a Algorithms
650 _ 2 |2 MeSH
|a Computer Simulation
650 _ 2 |2 MeSH
|a Diffusion
650 _ 2 |2 MeSH
|a Models, Chemical
650 _ 2 |2 MeSH
|a Suspensions
650 _ 2 |2 MeSH
|a Thermodynamics
650 _ 7 |0 0
|2 NLM Chemicals
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650 _ 7 |a J
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700 1 _ |a Ripoll, M.
|b 1
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|0 P:(DE-Juel1)130920
773 _ _ |a 10.1063/1.4723685
|g Vol. 136
|q 136
|0 PERI:(DE-600)1473050-9
|t The @journal of chemical physics
|v 136
|y 2012
|x 0021-9606
|p 204508
856 7 _ |u http://dx.doi.org/10.1063/1.4723685
856 4 _ |u https://juser.fz-juelich.de/record/21323/files/FZJ-21323.pdf
|y Published under German "Allianz" Licensing conditions on 2012-05-31. Available in OpenAccess from 2012-05-31
|z Published final document.
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913 1 _ |b Schlüsseltechnologien
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|v BioSoft: Makromolekulare Systeme und biologische Informationsverarbeitung
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913 2 _ |a DE-HGF
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|l BioSoft Fundamentals for future Technologies in the fields of Soft Matter and Life Sciences
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|v Functional Macromolecules and Complexes
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914 1 _ |y 2012
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