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@ARTICLE{Tappertzhofen:21890,
author = {Tappertzhofen, S. and Mündelein, H. and Valov, I. and
Waser, R.},
title = {{N}anoionic transport and electrochemical reactions in
resistively switching siicon dioxide},
journal = {Nanoscale},
volume = {4},
issn = {2040-3364},
address = {Cambridge},
publisher = {RSC Publ.},
reportid = {PreJuSER-21890},
pages = {3040 - 3043},
year = {2012},
note = {Record converted from VDB: 12.11.2012},
abstract = {The mobility of copper ions and redox reactions of Cu at
the interface with SiO(2) being directly attributed to the
resistive switching effect have been studied by cyclic
voltammetry (CV). The electrode kinetics of the Cu(z+)/Cu
redox reactions were analyzed suggesting the formation of
both Cu(+) and Cu(2+) species. The ion mobility shows an
unexpected strong dependence on the ion concentration
indicating ion-ion interactions typical for concentrated
solution conditions. Based on the standard reduction
potentials for Cu(z+)/Cu we identified partial
electrochemical redox reactions during oxidation and
reduction. The results contribute to a detailed
understanding of the resistive switching effect in
Cu/SiO(2)/Pt cells and provide insight into
electrochemically assisted diffusion of metal cations in
oxides in general.},
keywords = {Copper: chemistry / Electrochemical Techniques / Electrodes
/ Ions: chemistry / Kinetics / Nanotechnology /
Oxidation-Reduction / Platinum: chemistry / Silicon Dioxide:
chemistry / Ions (NLM Chemicals) / Platinum (NLM Chemicals)
/ Copper (NLM Chemicals) / Silicon Dioxide (NLM Chemicals) /
J (WoSType)},
cin = {PGI-7 / JARA-FIT},
ddc = {600},
cid = {I:(DE-Juel1)PGI-7-20110106 / $I:(DE-82)080009_20140620$},
pnm = {Grundlagen für zukünftige Informationstechnologien},
pid = {G:(DE-Juel1)FUEK412},
shelfmark = {Chemistry, Multidisciplinary / Nanoscience $\&$
Nanotechnology / Materials Science, Multidisciplinary /
Physics, Applied},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:22504836},
UT = {WOS:000303604000006},
doi = {10.1039/c2nr30413a},
url = {https://juser.fz-juelich.de/record/21890},
}