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000021907 084__ $$2WoS$$aEngineering, Electrical & Electronic
000021907 1001_ $$0P:(DE-Juel1)VDB5464$$aDittmann, R.$$b0$$uFZJ
000021907 245__ $$aScaling Potential of Local Redox Processes in Memristive SrTiO _{3} Thin-Film Devices
000021907 260__ $$aNew York, NY [u.a.]$$bInst.$$c2012
000021907 300__ $$a1979 - 1990
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000021907 440_0 $$023582$$aProceedings of the IEEE$$v100$$x0018-9219$$y6
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000021907 500__ $$aManuscript received September 15, 2010; revised September 7, 2011; accepted February 7, 2012. Date of publication April 24, 2012; date of current version May 10, 2012. This work was supported in part by the Deutsche Forschungsgemeinschaft (SFB 917).
000021907 520__ $$aIn this work, we address the following question: Where do the resistive switching processes take place in memristive thin-film devices of the single crystalline model material Fe-doped SrTiO3? We compare resistive switching induced by the tip of the atomic force microscope on the bare thin-film surface with the switching properties observed in memristive devices with Pt top electrode. In order to close the gap between these two approaches, we combine conductive-tip atomic force microscopy with a delamination technique to remove the top electrode of Fe-doped SrTiO3 metal-insulator-metal (MIM) structures to gain insight into the active switching interface with nanoscale lateral resolution. This enables us to prove the coexistence of a filamentary and area-dependent switching process with opposite switching polarities in the same sample. The spatially resolved analysis by transmission electron microscopy and photoelectron spectromicroscopy gives us some hints that the two switching types take place in device regions with different defect density and significant stoichiometry difference.
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000021907 65320 $$2Author$$aDevice scaling
000021907 65320 $$2Author$$amemristive device
000021907 65320 $$2Author$$aredox process
000021907 65320 $$2Author$$aresistive switching
000021907 65320 $$2Author$$atransition metal oxides
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000021907 7001_ $$0P:(DE-Juel1)VDB64025$$aMünstermann, R.$$b1$$uFZJ
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000021907 7001_ $$0P:(DE-Juel1)131022$$aWaser, R.$$b9$$uFZJ
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