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000021988 1001_ $$0P:(DE-Juel1)VDB102813$$aRogers, S.$$b0$$uFZJ
000021988 245__ $$aThe molecular origin of stress generation in worm-like micelles, using a rheo-SANS LAOS approach
000021988 260__ $$aCambridge$$bRoyal Society of Chemistry (RSC)$$c2012
000021988 300__ $$a3831 - 3839
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000021988 440_0 $$016881$$aSoft Matter$$v8$$x1744-683X$$y30
000021988 500__ $$aFinancial support by the German Research Foundation within SFB TR 6, and the European Network Nanodirect (grant no. NMP4-SL-2008-213948). The authors thank P. Ballesta for fruitful discussions.
000021988 520__ $$aWe combine large-amplitude oscillatory shear (LAOS) and time-resolved small angle neutron scattering (t-SANS) measurements on the dynamic response of a dispersion of surfactant worm-like micelles. By viewing the response as being the result of a sequence of physical processes, we observe new features of the system response. We identify three distinct frequency regimes including a high frequency Maxwell-like, a yielding, and a settled flow regime. For each regime we identify the molecular origins, on a Kuhn segment scale, of the stress response. We show the ability of the material to 'over-orient' pre-yielding, compared with stationary flow. Finally, we present a stress-orientation rule which is rate-based at low frequencies and strain-based at high frequencies.
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000021988 7001_ $$0P:(DE-HGF)0$$aKohlbrecher, J.$$b1
000021988 7001_ $$0P:(DE-Juel1)130797$$aLettinga, M.P.$$b2$$uFZJ
000021988 773__ $$0PERI:(DE-600)2191476-X$$a10.1039/c2sm25569c$$gVol. 8, p. 3831 - 3839$$p3831 - 3839$$q8<3831 - 3839$$tSoft matter$$v8$$x1744-683X$$y2012
000021988 8567_ $$uhttp://dx.doi.org/10.1039/c2sm25569c
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