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000022302 084__ $$2WoS$$aChemistry, Multidisciplinary
000022302 084__ $$2WoS$$aCrystallography
000022302 084__ $$2WoS$$aMaterials Science, Multidisciplinary
000022302 1001_ $$0P:(DE-HGF)0$$aMalaestean, I.L.$$b0
000022302 245__ $$aLinear, Zig-zag and Helical Cerium(III) Coordination Polymers
000022302 260__ $$aWashington, DC$$bACS Publ.$$c2012
000022302 300__ $$a1593 - 1602
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000022302 440_0 $$024841$$aCrystal Growth and Design$$v12$$y3
000022302 500__ $$3POF3_Assignment on 2016-02-29
000022302 500__ $$aWe thank Yutian Wang for collecting crystallographic data sets for compounds 1, 3, and S. Work at the Ames Laboratory was supported by the Department of Energy-Basic Energy Sciences under Contract No. DE-AC02-07CH11358.
000022302 520__ $$aFive novel one-dimensional cerium(III) carboxylate coordination polymers, [Ce(O2CCH2CHMe2)(3)(EtOH)(2)](n) (1), {[Ce(O2CCH2Me)(3)(H2O)]center dot 0.5(4,4'-bpy)}(n) (2; 4,4'-bpy = 4,4'-bipyridine), {[Ce-2(O2CCHMe2)(6)(H2O)(3)]}(n) (3), {[Ce-3(O2CCHMe2)(9)(nPrOH)(4)]}(n) (4), and {[Ce-3(O2CCHMe2)(9)(HO2CCHMe2)(2-)(H2O)(2)]center dot 2Me(2)CHCO(2)H}(n) (5), showcase the surprisingly consistent tendency of Ce(III) coordination network structures to adopt one-dimensional connection modes. The type of carboxylate as well as the reaction solvents determines the exact bridging versus end-on coordination modes for the carboxylates and, in turn, discriminate between linear, zigzag, and helical arrangements. Detailed magnetochemical analyses reveal pronounced single-ion effects and the expected weak antiferromagnetic coupling.
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000022302 7001_ $$0P:(DE-HGF)0$$aKutluca Alici, M.$$b1
000022302 7001_ $$0P:(DE-HGF)0$$aEllern, A.$$b2
000022302 7001_ $$0P:(DE-HGF)0$$avan Leusen, J.$$b3
000022302 7001_ $$0P:(DE-HGF)0$$aSchilder, H.$$b4
000022302 7001_ $$0P:(DE-HGF)0$$aSpeldrich, M.$$b5
000022302 7001_ $$0P:(DE-HGF)0$$aBaca, S.G.$$b6
000022302 7001_ $$0P:(DE-Juel1)VDB12080$$aKögerler, P.$$b7$$uFZJ
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000022302 8567_ $$uhttp://dx.doi.org/10.1021/cg2016337
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