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@ARTICLE{Donahue:22392,
      author       = {Donahue, N.M. and Henry, K.M. and Mentel, Th.F. and
                      Kiendler-Scharr, A. and Spindler, C. and Bohn, B. and
                      Brauers, Th. and Dorn, H.P. and Fuchs, H. and Tillmann, R.
                      and Wahner, A. and Saathoff, H. and Naumann, K.-H. and
                      Möhler, O. and Leisner, Th. and Müller, L. and Reinnig,
                      M.-C. and Hoffmann, T. and Salo, K. and Hallquist, M. and
                      Frosch, M. and Bilde, M. and Tritscher, T. and Barmet, P.
                      and Paraplan, A.P. and DeCarlo, P.F. and Dommen, J. and
                      Prevot, A.S.H. and Baltensperger, U.},
      title        = {{A}ging of biogenic secondary organic aerosol via gas-phase
                      {OH} radical reactions},
      journal      = {Proceedings of the National Academy of Sciences of the
                      United States of America},
      volume       = {109},
      number       = {34},
      issn         = {0027-8424},
      address      = {Washington, DC},
      publisher    = {Academy},
      reportid     = {PreJuSER-22392},
      pages        = {1-6},
      year         = {2012},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {The Multiple Chamber Aerosol Chemical Aging Study
                      (MUCHACHAS) tested the hypothesis that hydroxyl radical (OH)
                      aging significantly increases the concentration of
                      first-generation biogenic secondary organic aerosol (SOA).
                      OH is the dominant atmospheric oxidant, and MUCHACHAS
                      employed environmental chambers of very different designs,
                      using multiple OH sources to explore a range of chemical
                      conditions and potential sources of systematic error. We
                      isolated the effect of OH aging, confirming our hypothesis
                      while observing corresponding changes in SOA properties. The
                      mass increases are consistent with an existing gap between
                      global SOA sources and those predicted in models, and can be
                      described by a mechanism suitable for implementation in
                      those models.},
      keywords     = {Aerosols: chemistry / Atmosphere / Biogenesis / Free
                      Radicals / Hydroxyl Radical / Mass Spectrometry: methods /
                      Models, Chemical / Organic Chemicals: chemistry / Oxygen:
                      chemistry / Ozone / Reproducibility of Results / Solvents:
                      chemistry / Ultraviolet Rays / Aerosols (NLM Chemicals) /
                      Free Radicals (NLM Chemicals) / Organic Chemicals (NLM
                      Chemicals) / Solvents (NLM Chemicals) / Ozone (NLM
                      Chemicals) / Hydroxyl Radical (NLM Chemicals) / Oxygen (NLM
                      Chemicals)},
      cin          = {IEK-8},
      ddc          = {000},
      cid          = {I:(DE-Juel1)IEK-8-20101013},
      pnm          = {Atmosphäre und Klima},
      pid          = {G:(DE-Juel1)FUEK491},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:22869714},
      pmc          = {pmc:PMC3427056},
      UT           = {WOS:000308085200020},
      doi          = {10.1073/pnas.1115186109},
      url          = {https://juser.fz-juelich.de/record/22392},
}