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@ARTICLE{Rosenfeldt:22532,
author = {Rosenfeldt, S. and Lüdel, F. and Schulreich, C. and
Hellweg, T. and Radulescu, A. and Schmelz, J. and Schmalz,
H. and Harnau, L.},
title = {{P}atchy worm-like micelles: solution structure studied by
small-angle neutron scattering},
journal = {Physical Chemistry Chemical Physics},
volume = {14},
issn = {1463-9076},
address = {Cambridge},
publisher = {RSC Publ.},
reportid = {PreJuSER-22532},
pages = {12750 - 12756},
year = {2012},
note = {This work was supported by the German Science Foundation
(Collaborative Research Center 840, project A2). We thank
the Julich Center of Neutron Scattering (JCNS, Germany) for
financial travel support and for providing beamtime at the
KWS 1 instrument at FRM II in Munich, Germany.},
abstract = {Triblock terpolymers exhibit a rich self-organization
behavior including the formation of fascinating cylindrical
core-shell structures with a phase separated corona. After
crystallization-induced self-assembly of
polystyrene-block-polyethylene-block-poly(methyl
methacrylate) triblock terpolymers (abbreviated as SEMs =
Styrene-Ethylene-Methacrylates) from solution, worm-like
core-shell micelles with a patchy corona of polystyrene and
poly(methyl methacrylate) were observed by transmission
electron microscopy. However, the solution structure is
still a matter of debate. Here, we present a method to
distinguish in situ between a Janus-type (two faced) and a
patchy (multiple compartments) configuration of the corona.
To discriminate between both models the scattering intensity
must be determined mainly by one corona compartment.
Contrast variation in small-angle neutron scattering enables
us to focus on one compartment of the worm-like micelles.
The results validate the existence of the patchy structure
also in solution.},
keywords = {J (WoSType)},
cin = {ICS-1 / JCNS (München) ; Jülich Centre for Neutron
Science JCNS (München) ; JCNS-FRM-II / JCNS-1},
ddc = {540},
cid = {I:(DE-Juel1)ICS-1-20110106 /
I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-1-20110106},
pnm = {BioSoft: Makromolekulare Systeme und biologische
Informationsverarbeitung (FUEK505) / 544 - In-house Research
with PNI (POF2-544)},
pid = {G:(DE-Juel1)FUEK505 / G:(DE-HGF)POF2-544},
experiment = {EXP:(DE-MLZ)KWS1-20140101},
shelfmark = {Chemistry, Physical / Physics, Atomic, Molecular $\&$
Chemical},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:22880203},
UT = {WOS:000308101100008},
doi = {10.1039/c2cp41231d},
url = {https://juser.fz-juelich.de/record/22532},
}