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@ARTICLE{Sydoruk:22539,
author = {Sydoruk, V. A. and Xiang, D. and Vitusevich, S. A. and
Petrychuk, M. V. and Vladyka, A. and Zhang, Y. and
Offenhäusser, A. and Kochelap, V. A. and Belyaev, A. E. and
Mayer, D.},
title = {{N}oise and transport characterization of single molecular
break junctions with individual molecule},
journal = {Journal of applied physics},
volume = {112},
issn = {0021-8979},
address = {Melville, NY},
publisher = {American Institute of Physics},
reportid = {PreJuSER-22539},
pages = {014908},
year = {2012},
note = {Financial support from Helmholtz-CSC is gratefully
acknowledged.},
abstract = {We studied the noise spectra of molecule-free and
molecule-containing mechanically controllable break
junctions. Both types of junctions revealed typical 1/f
noise characteristics at different distances between the
contacts with square dependence of current noise power
spectral density on current. Additional Lorentzian-shape
(1/f(2)) noise components were recorded only when
nanoelectrodes were bridged by individual 1,4-benzenediamine
molecule. The characteristic frequency of the revealed
1/f(2) noise related to a single bridging molecule
correlates with the lock-in current amplitudes. The recorded
behavior of Lorentzian-shape noise component as a function
of current is interpreted as the manifestation of a dynamic
reconfiguration of molecular coupling to the metal
electrodes. We propose a phenomenological model that
correlates the charge transport via a single molecule with
the reconfiguration of its coupling to the metal electrodes.
Experimentally obtained results are in good agreement with
theoretical ones and indicate that coupling between the
molecule metal electrodes is important aspect that should be
taken into account. (C) 2012 American Institute of Physics.
[http://dx.doi.org/10.1063/1.4736558]},
keywords = {J (WoSType)},
cin = {ICS-8 / PGI-8 / JARA-FIT},
ddc = {530},
cid = {I:(DE-Juel1)ICS-8-20110106 / I:(DE-Juel1)PGI-8-20110106 /
$I:(DE-82)080009_20140620$},
pnm = {Grundlagen für zukünftige Informationstechnologien /
BioSoft: Makromolekulare Systeme und biologische
Informationsverarbeitung},
pid = {G:(DE-Juel1)FUEK412 / G:(DE-Juel1)FUEK505},
shelfmark = {Physics, Applied},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000306513400157},
doi = {10.1063/1.4736558},
url = {https://juser.fz-juelich.de/record/22539},
}