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@ARTICLE{DePasquale:22799,
author = {De Pasquale, C. and Marsala, V. and Berns, A.E. and
Valagussa, M. and Pozzi, A. and Alonzo, G. and Conte, P.},
title = {{F}ast field cycling {NMR} relaxometry characterization of
biochars obtained from an industrial thermochemical process},
journal = {Journal of soils and sediments},
volume = {12},
issn = {1439-0108},
address = {Landsberg},
publisher = {Ecomed Publ.},
reportid = {PreJuSER-22799},
pages = {1211 - 1221},
year = {2012},
note = {Record converted from VDB: 12.11.2012},
abstract = {Biochar has unique properties which make it a powerful tool
to increase soil fertility and to contribute to the decrease
of the amount of atmospheric carbon dioxide through the
mechanisms of C sequestration in soils. Chemical and
physical biochar characteristics depend upon the technique
used for its production and the biomass nature. For this
reason, biochar characterization is very important in order
to address its use either for agricultural or environmental
purposes.Three different biochars obtained from an
industrial gasification process were selected in order to
establish their chemical and physical peculiarities for a
possible use in agronomical practices. They were obtained by
charring residues from the wine-making industry (marc) and
from poplar and conifer forests. Routine analyses such as pH
measurements, elemental composition, and ash and metal
contents were performed together with the evaluation of the
cross-polarization magic angle spinning (CPMAS) C-13 NMR
spectra of all the biochar samples. Finally, relaxometry
properties of water-saturated biochars were retrieved in
order to obtain information on pore size distribution.All
the biochars revealed basic pH values due to their large
content of alkaline metals. The quality of CPMAS C-13 NMR
spectra, which showed the typical signal pattern for charred
systems, was not affected by the presence of paramagnetic
centers. Although paramagnetism was negligible for the
acquisition of solid state spectra, it was effective in some
of the relaxometry experiments. For this reason, no useful
information could be retrieved about water dynamics in marc
char. Conversely, both relaxograms and nuclear magnetic
resonance dispersion profiles of poplar and conifer chars
indicated that poplar char is richer in small-sized pores,
while larger pores appear to be characteristic for the
conifer char.This study showed the potential of relaxometry
in revealing chemical-physical information on industrially
produced biochar. This knowledge is of paramount importance
to properly direct biochar agronomical uses.},
keywords = {J (WoSType)},
cin = {IBG-3},
ddc = {550},
cid = {I:(DE-Juel1)IBG-3-20101118},
pnm = {Terrestrische Umwelt},
pid = {G:(DE-Juel1)FUEK407},
shelfmark = {Geosciences, Multidisciplinary / Soil Science},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000307519400002},
doi = {10.1007/s11368-012-0489-x},
url = {https://juser.fz-juelich.de/record/22799},
}