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000022814 1001_ $$0P:(DE-HGF)0$$aHong, H.B.$$b0
000022814 245__ $$aIn situ analysis of free radicals from the photodecomposition of hydrogen peroxide using a frequency-mixing magnetic detector
000022814 260__ $$aMelville, NY$$bAmerican Institute of Physics$$c2012
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000022814 440_0 $$0562$$aApplied Physics Letters$$v101$$x0003-6951$$y5
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000022814 500__ $$aThis research was supported financially by the Converging Research Center Program (2011K000677) and the World Class University (WCU) Program (R31-20029) through the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science and Technology, Republic of Korea.
000022814 520__ $$aWe present an analytical method for the real-time detection of free radicals from the photodecomposition (ultraviolet radiation, lambda = 254 nm) of hydrogen peroxide (H2O2) using frequency-mixing magnetic detection. We monitored the free radicals in situ without catalysts or probe molecules. Both water and H2O2 produced frequency-mixing signals under UV radiation, but the water signal was much weaker. The root mean square amplitude of the frequency-mixing signal was found to depend on the initial H2O2 concentration. Considering the physical properties of the reactants, the frequency-mixing signal is attributed to the generation of paramagnetic free radicals by the photodecomposition of H2O2. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.47427401
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000022814 7001_ $$0P:(DE-Juel1)128697$$aKrause, H.-J.$$b1$$uFZJ
000022814 7001_ $$0P:(DE-HGF)0$$aSong, K.$$b2
000022814 7001_ $$0P:(DE-HGF)0$$aChoi, C.-J.$$b3
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000022814 8567_ $$uhttp://dx.doi.org/10.1063/1.4742740
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