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000022839 084__ $$2WoS$$aPhysics, Multidisciplinary
000022839 1001_ $$0P:(DE-Juel1)VDB108913$$aRogers, S.A.$$b0$$uFZJ
000022839 245__ $$aRotational Diffusion of Spherical Colloids Close to a Wall
000022839 260__ $$aCollege Park, Md.$$bAPS$$c2012
000022839 300__ $$a098305
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000022839 440_0 $$04925$$aPhysical Review Letters$$v109$$x0031-9007
000022839 500__ $$aThe authors acknowledge financial support from the EU through FP7, project Nanodirect (Grant No. NMP4-SL-2008-213948). M. L. acknowledges support by the Foundation for Polish Science, which is co-financed by the European Union (EU)-European Regional Development Fund. B. C. acknowledges financial support from the Deutsche Forschungsgemeinschaft Grant No. SFB-TR6, "Physics of Colloidal Dispersions in External Fields," Project A1.
000022839 520__ $$aThere is currently no experimental technique available to probe spatially resolved rotational diffusion of nanoparticles in the vicinity of a wall. We present the first experimental study of rotational diffusion of small spherical colloids, using dynamic evanescent wave scattering. A setup is used where the wave vector components parallel and perpendicular to the wall can be varied independently, and an expression is derived for the first cumulant of the intensity correlation function in VH evanescent wave geometry for optically anisotropic spheres. The experimental results are in agreement with theoretical predictions that take particle-wall hydrodynamic interactions into account.
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000022839 7001_ $$0P:(DE-HGF)0$$aLisicki, M.$$b1
000022839 7001_ $$0P:(DE-HGF)0$$aCichocki, B.$$b2
000022839 7001_ $$0P:(DE-Juel1)130616$$aDhont, J.K.G.$$b3$$uFZJ
000022839 7001_ $$0P:(DE-Juel1)130789$$aLang, P.R.$$b4$$uFZJ
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000022839 8567_ $$uhttp://dx.doi.org/10.1103/PhysRevLett.109.098305
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