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@ARTICLE{Nair:23058,
author = {Nair, H. and Swain, D. and Hariharan, N. and Adiga, S. and
Narayana, C. and Elzabeth, S.},
title = {{G}riffiths phase-like behavior and spin-phonon coupling in
double perovskite {T}b2{N}i{M}n{O}6},
journal = {Journal of applied physics},
volume = {110},
issn = {0021-8979},
address = {Melville, NY},
publisher = {American Institute of Physics},
reportid = {PreJuSER-23058},
pages = {123919},
year = {2011},
note = {S.E. wishes to thank Department of Science and Technology,
India, for financial support through project grants.},
abstract = {The Griffiths phase-like features and the spin-phonon
coupling effects observed in Tb2NiMnO6 are reported. The
double perovskite compound crystallizes in monoclinic
P2(1)/n space group and exhibits a magnetic phase transition
at T-c similar to 111 K as an abrupt change in
magnetization. A negative deviation from ideal Curie-Weiss
law exhibited by 1/chi(T) curves and less-than-unity
susceptibility exponents from the power-law analysis of
inverse susceptibility are reminiscent of Griffiths
phase-like features. Arrott plots derived from magnetization
isotherms support the inhomogeneous nature of magnetism in
this material. The observed effects originate from
antiferromagnetic interactions that arise from inherent
disorder in the system. Raman scattering experiments display
no magnetic-order-induced phonon renormalization below Tc in
Tb2NiMnO6, which is different from the results observed in
other double perovskites and is correlated to the smaller
size of the rare earth. The temperature evolution of
full-width-at-half-maximum for the stretching mode at 645
cm(-1) presents an anomaly that coincides with the magnetic
transition temperature and signals a close connection
between magnetism and lattice in this material. (C) 2011
American Institute of Physics. [doi: 10.1063/1.3671674]},
keywords = {J (WoSType)},
cin = {PGI-4 / JCNS (München) ; Jülich Centre for Neutron
Science JCNS (München) ; JCNS-FRM-II / JCNS-2},
ddc = {530},
cid = {I:(DE-Juel1)PGI-4-20110106 /
I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-2-20110106},
pnm = {Grundlagen für zukünftige Informationstechnologien
(FUEK412) / 544 - In-house Research with PNI (POF2-544)},
pid = {G:(DE-Juel1)FUEK412 / G:(DE-HGF)POF2-544},
experiment = {EXP:(DE-MLZ)NOSPEC-20140101},
shelfmark = {Physics, Applied},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000298639800078},
doi = {10.1063/1.3671674},
url = {https://juser.fz-juelich.de/record/23058},
}