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@ARTICLE{Caciuc:23153,
author = {Caciuc, V. and Atodiresei, N. and Callsen, M. and Lazic, P.
and Blügel, S.},
title = {{A}b initio and semi-empirical van der {W}aals study of
graphene-boron nitride interaction from a molecular point of
view},
journal = {Journal of physics / Condensed matter},
volume = {24},
issn = {0953-8984},
address = {Bristol},
publisher = {IOP Publ.},
reportid = {PreJuSER-23153},
pages = {424214},
year = {2012},
note = {Record converted from VDB: 12.11.2012},
abstract = {We have performed a systematic semi-empirical and ab initio
van der Waals study to investigate the bonding mechanism of
benzene (C(6)H(6)), triazine (C(3)N(3)H(3)) and borazine
(B(3)N(3)H(6)) adsorbed on graphene and a single boron
nitride (BN) sheet. The two semi-empirical approaches used
to include the van der Waals (vdW) interactions in our
density functional theory (DFT) calculations suggest that
the strength of the molecule-surface interaction corresponds
to a strong physisorption with no net charge transfer
between the molecules and the corresponding substrates. This
observation is strengthened by the use of first-principles
non-local correlation vdW-DF functionals which provide a
sound physical basis to include vdW interactions in DFT
calculations. In particular we have employed two flavors of
vdW-DF functionals which enabled us to determine the role of
the non-local correlation effects in the molecule-surface
bonding mechanism which cannot be assessed by using only
semi-empirical vdW methods. Our study also reveals that the
strength of the molecule-surface interaction can be
influenced by the electronegativity of the B, C and N
atoms.},
cin = {PGI-1 / IAS-1 / JARA-FIT / JARA-SIM},
ddc = {530},
cid = {I:(DE-Juel1)PGI-1-20110106 / I:(DE-Juel1)IAS-1-20090406 /
$I:(DE-82)080009_20140620$ / I:(DE-Juel1)VDB1045},
pnm = {Grundlagen für zukünftige Informationstechnologien},
pid = {G:(DE-Juel1)FUEK412},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:23032913},
UT = {WOS:000309956300015},
doi = {10.1088/0953-8984/24/42/424214},
url = {https://juser.fz-juelich.de/record/23153},
}