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000023329 084__ $$2WoS$$aChemistry, Physical
000023329 1001_ $$0P:(DE-Juel1)144087$$aWang, Z.$$b0$$uFZJ
000023329 245__ $$aThermal Diffusion of Nucleotides
000023329 260__ $$aWashington, DC$$bSoc.$$c2012
000023329 300__ $$a7463 - 7469
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000023329 440_0 $$03694$$aJournal of Physical Chemistry B$$v116$$x1520-6106$$y25
000023329 500__ $$aWe appreciate many fruitful discussions with Dieter Braun and Pablo Blanco. We express our gratitude to Jan Dhont for his generous support. We thank Sabine Willbold for performing the NMR measurements and Doris Vollmer for her help with the micro calorimetry experiments. Financial support due to the Deutsche Forschungsgemeinschaft Grant Wi 1684 is gratefully acknowledged.
000023329 520__ $$aWe investigate the thermal diffusion behavior of aqueous solutions of nucleotides using an infrared thermal diffusion forced Rayleigh scattering (IR-TDFRS) setup. In this work we study 5 nucleotides: cyclic nucleotides adenosine and guanosine monophosphate, 5'-adenosine and 5'-cytidine monophosphate, and also adenosine diphosphate in water. The structures of nucleotides vary systematically, which results in different physical properties such as acidity, solubility, hydrophobicity, and melting point. We discuss the connection between the thermal diffusion behavior and the properties of the different nucleotides. Additionally, as in the case of the alkanes and monoscaccharides, we find a correlation between the thermal diffusion coefficient and the ratio of the thermal expansion coefficient and the kinematic viscosity.
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000023329 650_2 $$2MeSH$$aNucleotides: chemistry
000023329 650_2 $$2MeSH$$aThermal Diffusion
000023329 650_2 $$2MeSH$$aThermodynamics
000023329 650_2 $$2MeSH$$aWater: chemistry
000023329 650_7 $$00$$2NLM Chemicals$$aNucleotides
000023329 650_7 $$07732-18-5$$2NLM Chemicals$$aWater
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000023329 7001_ $$0P:(DE-Juel1)130773$$aKriegs, H.$$b1$$uFZJ
000023329 7001_ $$0P:(DE-Juel1)131034$$aWiegand, S.$$b2$$uFZJ
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