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@ARTICLE{Piotrowski:23567,
author = {Piotrowski, M. and Janowitz, T. and Kneifel, H.},
title = {{P}lant {C}-{N}-{H}ydrolases and the identification of a
plant {N}-{C}arbamoylputrescine amidohydrolase involved in
polyamine biosynthesis},
journal = {The journal of biological chemistry},
volume = {278},
issn = {0021-9258},
address = {Bethesda, Md.},
publisher = {Soc.},
reportid = {PreJuSER-23567},
pages = {1708 - 1712},
year = {2003},
note = {Record converted from VDB: 12.11.2012},
abstract = {A nitrilase-like protein from Arabidopsis thaliana (NLP1)
was expressed in Escherichia coli as a His(6)-tagged protein
and purified to apparent homogeneity by Ni(2+)-chelate
affinity chromatography. The purified enzyme showed
N-carbamoylputrescine amidohydrolase activity, an enzyme
involved in the biosynthesis of polyamines in plants and
bacteria. N-carbamoylputrescine amidohydrolase activity was
confirmed by identification of two of the three occurring
products, namely putrescine and ammonia. In contrast, no
enzymatic activity could be detected when applying various
compounds including nitriles, amines, and amides as well as
other N-carbamoyl compounds, indicating the specificity of
the enzyme for N-carbamoylputrescine. Like the homologous
beta-alanine synthases, NLP1 showed positive cooperativity
toward its substrate. The native enzyme had a molecular mass
of 279 kDa as shown by blue-native polyacrylamide gel
electrophoresis, indicating a complex of eight monomers.
Expression of the NLP1 gene was found in all organs
investigated, but it was not induced upon osmotic stress,
which is known to induce biosynthesis of putrescine. This is
the first report of cloning and expression of a plant
N-carbamoylputrescine amidohydrolase and the first time that
N-carbamoylputrescine amidohydrolase activity of a
recombinant protein could be shown in vitro. NLP1 is one of
the two missing links in the arginine decarboxylase pathway
of putrescine biosynthesis in higher plants.},
keywords = {Arabidopsis: enzymology / Biogenic Polyamines: biosynthesis
/ Blotting, Northern / Electrophoresis, Polyacrylamide Gel /
Mass Spectrometry / Phylogeny / Ureohydrolases: chemistry /
Ureohydrolases: genetics / Ureohydrolases: metabolism /
Biogenic Polyamines (NLM Chemicals) / N-carbamoylputrescine
hydrolase (NLM Chemicals) / Ureohydrolases (NLM Chemicals) /
J (WoSType)},
cin = {ICG-III},
ddc = {570},
cid = {I:(DE-Juel1)VDB49},
pnm = {Chemie und Dynamik der Geo-Biosphäre},
pid = {G:(DE-Juel1)FUEK257},
shelfmark = {Biochemistry $\&$ Molecular Biology},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:12435743},
UT = {WOS:000180462200046},
doi = {10.1074/jbc.M205699200},
url = {https://juser.fz-juelich.de/record/23567},
}