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@ARTICLE{KooLee:23904,
author = {Koo Lee, S. A. and Führ, F. and Wook Kwon, J. and Chang
Ahn, K.},
title = {{L}ong-term fate of the herbicide cinosulfuron in
lysimeters planted with rice over four consecutive years},
journal = {Chemosphere},
volume = {49},
issn = {0045-6535},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {PreJuSER-23904},
pages = {173 - 181},
year = {2002},
note = {Record converted from VDB: 12.11.2012},
abstract = {in order to elucidate the long-term fate of the
sulfonylurea herbicide cinosulfuron, the C-14-labelled
chemical was applied to a clay loam soil, encased in two
lysimeters, 22 days after rice (Oryza sativa L.)
transplanting, and rice plants were grown for four
consecutive years. Throughout the experimental period,
leaching through soil profiles, absorption and translocation
by rice plants, and distribution of C-14 by downward
movement in the soil layers were clarified. The total volume
of leachates collected through the lysimeter soil over the
four years amounted to 168 and 146 L in lysimeters I and 11,
respectively. The leachates contained $2.43\%$ and $2.99\%$
of the originally applied C-14-radioactivity, corresponding
to an average concentration of 0.29 and 0.41 mug/L as the
cinosulfuron equivalent in lysimeters I and II,
respectively. The total C-14-radioactivity translocated to
rice plants in the third and fourth year was $0.69\%$ and
$0.60\%$ (lysimeter 1), and $1.02\%$ and $0.84\%$ (lysimeter
11) of the C-14 applied, respectively. Larger amounts of
cinosulfuron equivalents $(0.54-0.75\%)$ remained in the
straw in the fourth year than in any other parts. The
C-14-radioactivities distributed down to a depth of 70 cm
after four years were $56.71-57.52\%$ of the C-14 applied,
indicating the continuous downward movement and degradation
of cinosulfuron in soil. The non-extractable residues were
more than $88\%$ of the soil radioactivity and some
$45-48\%$ of them was incorporated into the humin fraction.
The C-14-radioactivity partitioned into the aqueous phase
was nearly $30\%$ of the extractable 14C, suggesting
strongly that cinosulfuron was degraded into some polar
products during the experimental period. It was found out in
a supplemental investigation that flooding and constant
higher temperature enhanced mineralization of
[C-14]cinosulfuron to (CO2)-C-14 in soil, indicating the
possibility of chemical hydrolysis and microbial degradation
of the compound in the flooded lysimeter soil. (C) 2002
Published by Elsevier Science Ltd.},
keywords = {J (WoSType)},
cin = {ICG-IV},
ddc = {333.7},
cid = {I:(DE-Juel1)VDB50},
pnm = {Chemie und Dynamik der Geo-Biosphäre},
pid = {G:(DE-Juel1)FUEK257},
shelfmark = {Environmental Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000178062800008},
doi = {10.1016/S0045-6535(02)00191-1},
url = {https://juser.fz-juelich.de/record/23904},
}