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@ARTICLE{Arbe:24202,
author = {Arbe, A. and Colmenero, J. and Alvarez, F. and Monkenbusch,
M. and Richter, D. and Farago, B. and Frick, K. H.},
title = {{N}on-{G}aussian nature of the alpha-relaxation of
glass-forming polyisoprene},
journal = {Physical review letters},
volume = {89},
issn = {0031-9007},
address = {College Park, Md.},
publisher = {APS},
reportid = {PreJuSER-24202},
pages = {245701},
year = {2002},
note = {Record converted from VDB: 12.11.2012},
abstract = {We report quasielastic neutron scattering experiments
exploring the alpha relaxation in polyisoprene over an
unprecedented range in momentum transfer. Corroborating and
validating earlier molecular dynamics simulations, the
measurements reveal a crossover from a Gaussian regime of
sublinear diffusion to a strongly non-Gaussian regime at
short distances. We show that a consistent interpretation in
terms of a distribution of finite jumps underlying the alpha
process is possible. This model leads to a time-dependent
non-Gaussian parameter exhibiting all features revealed so
far from various simulations.},
keywords = {J (WoSType)},
cin = {IFF-NST},
ddc = {550},
cid = {I:(DE-Juel1)VDB34},
pnm = {Kondensierte Materie},
pid = {G:(DE-Juel1)FUEK242},
shelfmark = {Physics, Multidisciplinary},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000179484700027},
doi = {10.1103/PhysRevLett.89.245701},
url = {https://juser.fz-juelich.de/record/24202},
}