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000255635 1001_ $$0P:(DE-Juel1)130679$$aGupta, Sudipta$$b0
000255635 245__ $$aValidity of the Stokes-Einstein Relation in Soft Colloids up to the Glass Transition
000255635 260__ $$aCollege Park, Md.$$bAPS$$c2015
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000255635 520__ $$aWe investigate the dynamics of kinetically frozen block copolymer micelles of different softness across a wide range of particle concentrations, from the fluid to the onset of glassy behavior, through a combination of rheology, dynamic light scattering, and pulsed field gradient NMR spectroscopy. We additionally perform Brownian dynamics simulations based on an ultrasoft coarse-grained potential, which are found to be in quantitative agreement with experiments, capturing even the very details of dynamic structure factors S(Q,t) on approaching the glass transition. We provide evidence that for these systems the Stokes-Einstein relation holds up to the glass transition; given that it is violated for dense suspensions of hard colloids, our findings suggest that its validity is an intriguing signature of ultrasoft interactions.
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000255635 7001_ $$0P:(DE-Juel1)130986$$aStellbrink, Jörg$$b1
000255635 7001_ $$0P:(DE-HGF)0$$aZaccarelli, Emanuela$$b2
000255635 7001_ $$0P:(DE-HGF)0$$aLikos, Christos N.$$b3
000255635 7001_ $$0P:(DE-HGF)0$$aCamargo, Manuel$$b4$$eCorresponding author
000255635 7001_ $$0P:(DE-Juel1)130719$$aHolmqvist, Peter$$b5
000255635 7001_ $$0P:(DE-Juel1)130501$$aAllgaier, J.$$b6
000255635 7001_ $$0P:(DE-Juel1)131036$$aWillner, Lutz$$b7
000255635 7001_ $$0P:(DE-Juel1)130917$$aRichter, Dieter$$b8
000255635 773__ $$0PERI:(DE-600)1472655-5$$a10.1103/PhysRevLett.115.128302$$gVol. 115, no. 12, p. 128302$$n12$$p128302$$tPhysical review letters$$v115$$x1079-7114$$y2015
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