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@ARTICLE{Braun:255641,
author = {Braun, Anika and Klumpp, Erwin and Azzam, Rafig and Neukum,
Christoph},
title = {{T}ransport and deposition of stabilized engineered silver
nanoparticles in water saturated loamy sand and silty loam},
journal = {The science of the total environment},
volume = {535},
issn = {0048-9697},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2015-05775},
pages = {102 - 112},
year = {2015},
abstract = {It is considered inevitable that the increasing production
and application of engineered nanoparticles will lead to
their release into the environment. However, the behavior of
these materials under environmentally relevant conditions is
still only poorly understood. In this study the transport
and deposition behavior of engineered surfactant stabilized
silver nanoparticles (AgNPs) in water saturated porous media
was investigated in transport experiments with glass beads
as reference porous medium and in two natural soils under
various hydrodynamic and hydrochemical conditions. The
transport and retention processes of AgNPs in the porous
media were elucidated by inverse modeling and possible
particle size changes occurring during the transport through
the soil matrix were analyzed with flow field-flow
fractionation (FlFFF). A high mobility of AgNPs was observed
in loamy sand under low ionic strength (IS) conditions and
at high flow rates. The transport was inhibited at low flow
rates, at higher IS, in the presence of divalent cations and
in a more complex, fine-grained silty loam. The slight
decrease of the mean particle size of the AgNPs in almost
all experiments indicates size selective filtration
processes and enables the exclusion of homoaggregation
processes.},
cin = {IBG-3},
ddc = {333.7},
cid = {I:(DE-Juel1)IBG-3-20101118},
pnm = {255 - Terrestrial Systems: From Observation to Prediction
(POF3-255)},
pid = {G:(DE-HGF)POF3-255},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000360291100013},
doi = {10.1016/j.scitotenv.2014.12.023},
url = {https://juser.fz-juelich.de/record/255641},
}