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@ARTICLE{Maeda:255866,
      author       = {Maeda, Kousaku and Shinyashiki, Naoki and Yagihara, Shin
                      and Wiegand, Simone and Kita, Rio},
      title        = {{L}udwig-{S}oret effect of aqueous solutions of ethylene
                      glycol oligomers, crown ethers, and glycerol: {T}emperature,
                      molecular weight, and hydrogen bond effect},
      journal      = {The journal of chemical physics},
      volume       = {143},
      number       = {12},
      issn         = {1089-7690},
      address      = {Melville, NY},
      publisher    = {American Institute of Physics},
      reportid     = {FZJ-2015-05972},
      pages        = {124504 -},
      year         = {2015},
      abstract     = {The thermal diffusion, also called the Ludwig-Soret effect,
                      of aqueous solutions of ethylene glycol oligomers, crown
                      ethers, and glycerol are investigated as a function of
                      temperature by Thermal Diffusion Forced Rayleigh Scattering
                      (TDFRS). The Soret coefficient, $S_{\rm{T}}$, and the
                      thermal diffusion coefficient, $D_{\rm{T}}$, show a linear
                      temperature dependence for all studied compounds in the
                      investigated temperature range. The magnitudes and the
                      slopes of $S_{\rm{T}}$ and $D_{\rm{T}}$ vary with the
                      chemical structure of the solute molecules. All studied
                      molecules contain ether and/or hydroxyl groups, which can
                      act as acceptor or donor to form hydrogen bonds,
                      respectively. By introducing the number of donor and
                      acceptor sites of each solute molecule, we can express their
                      hydrogen bond capability. $S_{\rm{T}}$ and $D_{\rm{T}}$ can
                      be described by an empirical equation depending on the
                      difference of donor minus acceptors sites and the molecular
                      weight of the solute molecule.},
      cin          = {ICS-3},
      ddc          = {540},
      cid          = {I:(DE-Juel1)ICS-3-20110106},
      pnm          = {551 - Functional Macromolecules and Complexes (POF3-551)},
      pid          = {G:(DE-HGF)POF3-551},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000362568100034},
      doi          = {10.1063/1.4931115},
      url          = {https://juser.fz-juelich.de/record/255866},
}