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@ARTICLE{Riest:255991,
      author       = {Riest, Jonas and Naegele, Gerhard},
      title        = {{S}hort-time dynamics in dispersions with competing
                      short-range attraction and long-range repulsion},
      journal      = {Soft matter},
      volume       = {11},
      number       = {48},
      issn         = {1744-6848},
      address      = {London},
      publisher    = {Royal Soc. of Chemistry},
      reportid     = {FZJ-2015-06047},
      pages        = {9273-9280},
      year         = {2015},
      abstract     = {Dynamic clustering of globular Brownian particles in
                      dispersions exhibiting competing short-range attraction and
                      long-range repulsion (SALR) such as low-salinity protein
                      solutions has gained a lot of interest over the past few
                      years. While the structure of the various cluster phases has
                      been intensely explored, little is known about the dynamics
                      of SALR systems. We present the first systematic theoretical
                      study of short-time diffusion and rheological transport
                      properties of two-Yukawa potential SALR systems in the
                      single-particle dominated dispersed-fluid phase, using
                      semi-analytic methods where the salient hydrodynamic
                      interactions are accounted for. We show that the dynamics
                      has unusual features compared to reference systems with pure
                      repulsion or attraction. Results are discussed for the
                      hydrodynamic function characterizing short-time diffusion
                      that reveals an intermediate-range-order (cluster) peak,
                      self-diffusion and sedimentation coefficients, and
                      high-frequency viscosity. As important applications, we
                      discuss the applicability of two generalized
                      Stokes–Einstein relations, and assess the wavenumber range
                      required for the determination of self-diffusion in a
                      dynamic scattering experiment.},
      cin          = {ICS-3},
      ddc          = {530},
      cid          = {I:(DE-Juel1)ICS-3-20110106},
      pnm          = {551 - Functional Macromolecules and Complexes (POF3-551)},
      pid          = {G:(DE-HGF)POF3-551},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000365908000005},
      doi          = {10.1039/C5SM02099A},
      url          = {https://juser.fz-juelich.de/record/255991},
}