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@ARTICLE{Paik:256223,
author = {Paik, Hanjong and Moyer, Jarrett A. and Spila, Timothy and
Tashman, Joshua W. and Mundy, Julia A. and Freeman, Eugene
and Shukla, Nikhil and Lapano, Jason M. and Engel-Herbert,
Roman and Zander, Willi and Schubert, Jürgen and Muller,
David A. and Datta, Suman and Schiffer, Peter and Schlom,
Darrell G.},
title = {{T}ransport properties of ultra-thin {VO}2 films on (001)
{T}i{O}2 grown by reactive molecular-beam epitaxy},
journal = {Applied physics letters},
volume = {107},
number = {16},
issn = {1077-3118},
address = {Melville, NY},
publisher = {American Inst. of Physics},
reportid = {FZJ-2015-06199},
pages = {163101 -},
year = {2015},
abstract = {We report the growth of (001)-oriented VO2 films as thin as
1.5 nm with abrupt and reproduciblemetal-insulator
transitions (MIT) without a capping layer. Limitations to
the growth of thinnerfilms with sharp MITs are discussed,
including the Volmer-Weber type growth mode due to thehigh
energy of the (001) VO2 surface. Another key limitation is
interdiffusion with the (001) TiO2substrate, which we
quantify using low angle annular dark field scanning
transmission electronmicroscopy in conjunction with electron
energy loss spectroscopy. We find that controlling
islandcoalescence on the (001) surface and minimization of
cation interdiffusion by using a low growthtemperature
followed by a brief anneal at higher temperature are crucial
for realizing ultrathin VO2films with abrupt MIT behavior.
VC 2015 AIP Publishing LLC.},
cin = {PGI-9 / JARA-FIT},
ddc = {530},
cid = {I:(DE-Juel1)PGI-9-20110106 / $I:(DE-82)080009_20140620$},
pnm = {521 - Controlling Electron Charge-Based Phenomena
(POF3-521)},
pid = {G:(DE-HGF)POF3-521},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000363781900023},
doi = {10.1063/1.4932123},
url = {https://juser.fz-juelich.de/record/256223},
}