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@INPROCEEDINGS{Wiegand:256303,
author = {Wiegand, Simone and Afanasenkau, Dzmitry and Wang, Zilin
and Buitenhuis, Johan and Dhont, Jan K.G.},
title = {{T}hermophoresis in {S}oft {M}atter {S}ystems},
school = {Uni. Cavite, Philippines},
reportid = {FZJ-2015-06267},
year = {2015},
abstract = {Thermophoresis or Thermal diffusion, which is also known as
the Ludwig–Soret effect, is the phenomenon where mass
transport is induced by a temperature gradient in a
multi-component system. So far there is only a limited
microscopic understanding for fluids. In the recent years
the « heat of transfer » concept has been successfully
applied to non-polar systems, but in aqueous systems the
situations is more complicated due to charge effects and
strong specific cross interactions so that this concept
fails. It turns out that this simple non-equilibrium
environment created by a temperature gradient can be
successfully employed to monitor for example the reaction
kinetics of large proteins with small substrate molecules,
which play an important role in living organisms and drug
development. The strong sensitivity of the proteins and
other water soluble biomolecules is probably caused by a
change in the hydration layer, which is influenced by subtle
conformation changes induced by the binding of the substrate
molecule. To get a better understanding of these phenomena
we investigated systematically various small molecules,
microemulsions and colloids by a holographic grating method
called infrared thermal diffusion forced Rayleigh scattering
(IR-TDFRS). Looking at the various systems we can identify
certain rules of thumb which will be discussed. Open
questions such as the molecular size dependence of the
thermal diffusion coefficient and its relation with the
interfacial tension and charge effects are
considered.Finally we discuss how thermophoresis might be
used in the near future as an alternative strategy to design
synthetic microswimmers, micromotors, or micropumps, which
have become promising tools in the field of microfluidics.
We give an outlook how locally controlled temperature
gradients at very small scales, allow the fabrication of
lab-on-chip devices, which can be used to manipulate
synthetic and biological colloids. Keywords: Thermophoresis,
colloids, aqueous mixtures, holographic grating technique,
microfluidic},
month = {Oct},
date = {2015-10-22},
organization = {17th SPVM National Physics Conference,
Cavite (Philippines), 22 Oct 2015 - 24
Oct 2015},
subtyp = {Plenary/Keynote},
cin = {ICS-3},
cid = {I:(DE-Juel1)ICS-3-20110106},
pnm = {551 - Functional Macromolecules and Complexes (POF3-551)},
pid = {G:(DE-HGF)POF3-551},
typ = {PUB:(DE-HGF)6},
url = {https://juser.fz-juelich.de/record/256303},
}