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@ARTICLE{Amelung:256540,
author = {Amelung, Wulf and Antar, P. and Kleeberg, I. and Oelmann,
Y. and Lücke, Andreas and Alt, F. and Lewandowski, Hans and
Pätzold, S. and Barej, J. A. M.},
title = {{T}he δ$_{18}${O} signatures of {HC}l-extractable soil
phosphates: methodological challenges and evidence of the
cycling of biological {P} in arable soil},
journal = {European journal of soil science},
volume = {66},
number = {6},
issn = {0022-4588},
address = {Oxford [u.a.]},
publisher = {Wiley-Blackwell},
reportid = {FZJ-2015-06424},
pages = {965-972},
year = {2015},
abstract = {Soil phosphates exchange oxygen atoms rapidly with soil
water once recycled by intracellular enzymes, thereby
approaching an equilibrium δ18OP signature that depends on
ambient temperature and the δ18OW signature of soil water.
We hypothesized that in the topsoil, phosphates reach this
equilibrium δ18OP signature even if amended by different
fertilizers. In the subsoil, however, there might be
phosphates with a smaller δ18OP value than that represented
by the isotopic equilibrium value, a condition that could
exist in the case of limited biological P cycling only. We
tested these hypotheses for the HCl-extractable P pool of
the Hedley fractionation scheme of arable soil in Germany,
which integrates over extended time-scales of the soil P
cycle. We sampled several types of fertilizer, the surface
soil that received these fertilizer types and composites
from a Haplic Luvisol depth profile under long-term
agricultural practice. Organic fertilizers had significantly
smaller δ18OP values than mineral fertilizers.
Intriguingly, the fields fertilized organically also tended
to have smaller δ18OP signatures than other types of
surface soil, which calls into question full isotopic
equilibrium at all sites. At depths below 50 cm, the soil
δ18OP values were even depleted relative to the values
calculated for isotopic equilibrium. This implies that
HCl-extractable phosphates in different soil horizons are of
different origins. In addition, it supports the assumption
that biological cycling of P by intracellular microbial
enzymes might have been relatively inefficient in the deeper
subsoil. At depths of 50–80 cm, there was a transition
zone of declining δ18OP values, which might be regarded as
the first evidence that the degree of biological P cycling
changed at this depth interval},
cin = {IBG-3},
ddc = {630},
cid = {I:(DE-Juel1)IBG-3-20101118},
pnm = {255 - Terrestrial Systems: From Observation to Prediction
(POF3-255)},
pid = {G:(DE-HGF)POF3-255},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000364312500001},
doi = {10.1111/ejss.12288},
url = {https://juser.fz-juelich.de/record/256540},
}