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@ARTICLE{Eiberger:256608,
      author       = {Eiberger, Jan and Wilkner, Kai and Reetz, Corinna and
                      Sebold, Doris and Jordan, Natividad and de Graaff, Marijke
                      and Meulenberg, Wilhelm Albert and Stöver, Detlev and Bram,
                      Martin},
      title        = {{I}nfluence of coal power plant exhaust gas on the
                      structure and performance of ceramic nanostructured gas
                      separation membranes},
      journal      = {International journal of greenhouse gas control},
      volume       = {43},
      issn         = {1750-5836},
      address      = {New York, NY [u.a.]},
      publisher    = {Elsevier},
      reportid     = {FZJ-2015-06475},
      pages        = {46 - 56},
      year         = {2015},
      abstract     = {In this work, we investigate the effect of coal power plant
                      exhaust gas on amino-modified mesoporous ceramic membranes.
                      The testing of ceramic membranes in the flue gas of
                      coal-fired power plants represents a new approach, as
                      testing under simulated flue gas conditions has already been
                      undertaken, but not yet during direct exposure to exhaust
                      gas. Flue gas exposure trials were carried out at a
                      lignite-fueled power plant and a hard-coal-fueled power
                      plant. Most experiments were conducted using a test rig
                      designed to bring planar membrane samples in direct contact
                      with unconditioned flue gas in the exhaust gas channel.
                      Another test rig was designed to test membrane modules with
                      pre-treated flue gas. The tested membranes had an
                      asymmetrical structure consisting of a macroporous α-Al2O3
                      support coated with a mesoporous γ-Al2O3 or 8YSZ
                      interlayer. The microporous functional top layer was made of
                      amino-functionalized silica. The tests revealed different
                      degradation mechanisms such as gypsum/fly ash deposition on
                      the membrane surface, pore blocking by water condensation,
                      chemical reactions and phase transformation. A detailed
                      analysis was carried out to evaluate their impact on the
                      membrane in order to assess membrane stability under real
                      conditions. The suitability of these membranes for this
                      application is critically discussed and an improved mode of
                      membrane operation is proposed.},
      cin          = {IEK-1},
      ddc          = {333.7},
      cid          = {I:(DE-Juel1)IEK-1-20101013},
      pnm          = {113 - Methods and Concepts for Material Development
                      (POF3-113)},
      pid          = {G:(DE-HGF)POF3-113},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000367110200005},
      doi          = {10.1016/j.ijggc.2015.10.005},
      url          = {https://juser.fz-juelich.de/record/256608},
}