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@ARTICLE{MartnezGalera:256626,
author = {Martínez-Galera, A. J. and Schröder, U. A. and Huttmann,
F. and Jolie, W. and Craes, F. and Busse, C. and Caciuc, V.
and Atodiresei, N. and Blügel, S. and Michely, T.},
title = {{O}xygen orders differently under graphene: new
superstructures on {I}r(111)},
journal = {Nanoscale},
volume = {8},
number = {4},
issn = {2040-3372},
address = {Cambridge},
publisher = {RSC Publ.},
reportid = {FZJ-2015-06489},
pages = {1932-1943},
year = {2016},
abstract = {Using scanning tunneling microscopy, the oxygen adsorbate
superstructures on bare Ir(111) are identified and compared
to the ones formed by intercalation in between graphene and
the Ir(111) substrate. For bare Ir(111) we observe O-(2 ×
2) and O-(2 × 1) structures, thereby clarifying a
persistent uncertainty about the existence of these
structures and the role of defects for their stability. For
the case of graphene-covered Ir(111), oxygen intercalation
superstructures can be imaged through the graphene monolayer
by choosing proper tunneling conditions. Depending on the
pressure, temperature and duration of O2 exposure as well as
on the graphene morphology, O-(2 × 2),
O-(√3×√3)-R30°, O-(2 × 1) and O-(2√3 ×
2√3)-R30° superstructures with respect to Ir(111) are
observed under the graphene cover. Two of these structures,
the O-(√3 × √3)-R30° and the (2√3 × 2√3)-R30°
structure are only observed when the graphene layer is on
top. Phase coexistence and formation conditions of the
intercalation structures between graphene and Ir(111) are
analyzed. The experimental results are compared to density
functional theory calculations including dispersive forces.
The existence of these phases under graphene and their
absence on bare Ir(111) are discussed in terms of possible
changes in the adsorbate-substrate interaction due to the
presence of the graphene cover.},
cin = {IAS-1 / PGI-1 / JARA-FIT},
ddc = {600},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106 /
$I:(DE-82)080009_20140620$},
pnm = {142 - Controlling Spin-Based Phenomena (POF3-142) / 143 -
Controlling Configuration-Based Phenomena (POF3-143)},
pid = {G:(DE-HGF)POF3-142 / G:(DE-HGF)POF3-143},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000368860900021},
doi = {10.1039/C5NR04976H},
url = {https://juser.fz-juelich.de/record/256626},
}