001     25855
005     20180210122529.0
024 7 _ |2 DOI
|a 10.1016/S0039-6028(02)01554-6
024 7 _ |2 WOS
|a WOS:000176584000014
037 _ _ |a PreJuSER-25855
041 _ _ |a eng
082 _ _ |a 540
084 _ _ |2 WoS
|a Chemistry, Physical
084 _ _ |2 WoS
|a Physics, Condensed Matter
100 1 _ |a Bombis, C.
|b 0
|u FZJ
|0 P:(DE-Juel1)VDB8642
245 _ _ |a Absolute surface free energies of Pb
260 _ _ |a Amsterdam
|b Elsevier
|c 2002
300 _ _ |a 83 - 96
336 7 _ |a Journal Article
|0 PUB:(DE-HGF)16
|2 PUB:(DE-HGF)
336 7 _ |a Output Types/Journal article
|2 DataCite
336 7 _ |a Journal Article
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|2 EndNote
336 7 _ |a ARTICLE
|2 BibTeX
336 7 _ |a JOURNAL_ARTICLE
|2 ORCID
336 7 _ |a article
|2 DRIVER
440 _ 0 |a Surface Science
|x 0039-6028
|0 5673
|v 511
500 _ _ |a Record converted from VDB: 12.11.2012
520 _ _ |a Three-dimensional (3D) equilibrium crystal shapes (ECS) of Pb are utilized for the first time to determine absolute surface free energies via a quantitative evaluation of the measured ECS and published values of step free energies of vicinal (1 1 1) surfaces. 3D images of Pb crystallites are obtained by scanning tunneling microscopy at 323-393 K. Line scans through high symmetry <1 1 0> azimuths are transformed into an anisotropic relative surface free energy, gamma(theta, T). The absolute surface free energy of Pb(1 1 1) is obtained from the limiting slopes, df(theta, T)/d tan theta, of the orientation dependent f(theta, T) gamma(theta, T)/ cos theta at the boundaries of the (1 1 1) facet, located at theta = 0degrees. This value is 25.7 +/- 1.4 meV/Angstrom(2) or 440 +/- 22 mJ/m(2). Absolute surface free energies of other low-index orientations, such as (1 0 0), (1 1 0) etc. are calculated from the relative anisotropy of gamma(theta)/gamma(1 1 1). It is found that surface free energies of orientation (h k l), expressed in meV/atom, scale with the number of bonds broken in forming such a surface. Free energies of steps bounding other facets, such as (1 0 0), (1 1 0), (1 1 2), (1 1 3) and (2 2 1), are evaluated in the [0 1 (1) over bar] zone, using the corresponding facet radii and the absolute surface free energies of those facets. (C) 2002 Published by Elsevier Science B.V.
536 _ _ |a Kondensierte Materie
|c M02
|2 G:(DE-HGF)
|0 G:(DE-Juel1)FUEK242
|x 0
588 _ _ |a Dataset connected to Web of Science
650 _ 7 |a J
|2 WoSType
653 2 0 |2 Author
|a equilibrium thermodynamics and statistical mechanics
653 2 0 |2 Author
|a scanning tunneling microscopy
653 2 0 |2 Author
|a surface energy
653 2 0 |2 Author
|a surface structure, morphology, roughness, and topography
653 2 0 |2 Author
|a lead
700 1 _ |a Emundts, A.
|b 1
|u FZJ
|0 P:(DE-Juel1)VDB5552
700 1 _ |a Nowicki, M.
|b 2
|u FZJ
|0 P:(DE-Juel1)VDB5549
700 1 _ |a Bonzel, D. I.
|b 3
|u FZJ
|0 P:(DE-Juel1)VDB5490
773 _ _ |a 10.1016/S0039-6028(02)01554-6
|g Vol. 511, p. 83 - 96
|p 83 - 96
|q 511<83 - 96
|0 PERI:(DE-600)1479030-0
|t Surface science
|v 511
|y 2002
|x 0039-6028
909 C O |o oai:juser.fz-juelich.de:25855
|p VDB
913 1 _ |k M02
|v Kondensierte Materie
|l Kondensierte Materie
|b Materie
|0 G:(DE-Juel1)FUEK242
|x 0
914 1 _ |y 2002
915 _ _ |0 StatID:(DE-HGF)0010
|a JCR/ISI refereed
920 1 _ |k ISG-3
|l Institut für Grenzflächen und Vakuumtechnologien
|d 31.12.2006
|g ISG
|0 I:(DE-Juel1)VDB43
|x 0
970 _ _ |a VDB:(DE-Juel1)17232
980 _ _ |a VDB
980 _ _ |a ConvertedRecord
980 _ _ |a journal
980 _ _ |a I:(DE-Juel1)PGI-3-20110106
980 _ _ |a UNRESTRICTED
981 _ _ |a I:(DE-Juel1)PGI-3-20110106


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