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000026705 084__ $$2WoS$$aChemistry, Multidisciplinary
000026705 1001_ $$0P:(DE-HGF)0$$aSilin, F. H.$$b0
000026705 245__ $$aThe role of surface free energy on the formation of hybrid bilayer membranes
000026705 260__ $$aWashington, DC$$bAmerican Chemical Society$$c2002
000026705 300__ $$a14676
000026705 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article
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000026705 440_0 $$08502$$aJournal of the American Chemical Society$$v124$$x0002-7863
000026705 500__ $$aRecord converted from VDB: 12.11.2012
000026705 520__ $$aThe interaction of small phospholipid vesicles with well-characterized surfaces has been studied to assess the effect of the surface free energy of the underlying monolayer on the formation of phospholipid/alkanethiol hybrid bilayer membranes (HBMs). The surface free energy was changed in a systematic manner using single-component alkanethiol monolayers and monolayers of binary mixtures of thiols. The binary surfaces were prepared on gold by self-assembly from binary solutions of the thiols HS-(CH(2))(n)()-X (n = 11, X = CH(3) or OH) in THF. Surface plasmon resonance (SPR), electrical capacitance, and atomic force microscopy (AFM) measurements were used to characterize the interaction of palmitoyl,oleoyl-phosphatidylcholine (POPC) vesicles with the surfaces. For all surfaces examined, it appears that the polar part of surface energy influences the nature of the POPC assembly that associates with the surface. Comparison of optical, capacitance, and AFM data suggests that vesicles can remain intact or partially intact even at surfaces with a contact angle with water of close to 100 degrees. In addition, comparison of the alkanethiols of different chain lengths and the fluorinated compound HS-(CH(2))(2)-(CF(2))(8)-CF(3) that characterize with a low value of the polar part of the surface energy suggests that the quality of the underlying monolayer in terms of number of defects has a significant influence on the packing density of the resulting HBM layer.
000026705 536__ $$0G:(DE-Juel1)FUEK252$$2G:(DE-HGF)$$aMaterialien, Prozesse und Bauelemente für die  Mikro- und Nanoelektronik$$cI01$$x0
000026705 588__ $$aDataset connected to Web of Science, Pubmed
000026705 650_2 $$2MeSH$$aAdsorption
000026705 650_2 $$2MeSH$$aAlkanes: chemistry
000026705 650_2 $$2MeSH$$aElectric Capacitance
000026705 650_2 $$2MeSH$$aHydrocarbons, Fluorinated: chemistry
000026705 650_2 $$2MeSH$$aKinetics
000026705 650_2 $$2MeSH$$aLipid Bilayers: chemistry
000026705 650_2 $$2MeSH$$aMembranes: chemistry
000026705 650_2 $$2MeSH$$aMicroscopy, Atomic Force
000026705 650_2 $$2MeSH$$aPhosphatidylcholines: chemistry
000026705 650_2 $$2MeSH$$aSulfhydryl Compounds: chemistry
000026705 650_2 $$2MeSH$$aSurface Plasmon Resonance
000026705 650_2 $$2MeSH$$aSurface Properties
000026705 650_2 $$2MeSH$$aThermodynamics
000026705 650_7 $$00$$2NLM Chemicals$$aAlkanes
000026705 650_7 $$00$$2NLM Chemicals$$aHydrocarbons, Fluorinated
000026705 650_7 $$00$$2NLM Chemicals$$aLipid Bilayers
000026705 650_7 $$00$$2NLM Chemicals$$aPhosphatidylcholines
000026705 650_7 $$00$$2NLM Chemicals$$aSulfhydryl Compounds
000026705 650_7 $$0112-40-3$$2NLM Chemicals$$an-dodecane
000026705 650_7 $$06753-55-5$$2NLM Chemicals$$a1-palmitoyl-2-oleoylphosphatidylcholine
000026705 650_7 $$2WoSType$$aJ
000026705 7001_ $$0P:(DE-HGF)0$$aWieder, H.$$b1
000026705 7001_ $$0P:(DE-HGF)0$$aWoodward, J. T.$$b2
000026705 7001_ $$0P:(DE-HGF)0$$aValincius, G.$$b3
000026705 7001_ $$0P:(DE-Juel1)128713$$aOffenhäusser, A.$$b4$$uFZJ
000026705 7001_ $$0P:(DE-Juel1)VDB11929$$aPlant, A. L.$$b5$$uFZJ
000026705 773__ $$0PERI:(DE-600)1472210-0$$a10.1021/ja026585+$$gVol. 124, p. 14676$$p14676$$q124<14676$$tJournal of the American Chemical Society$$v124$$x0002-7863$$y2002
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