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@ARTICLE{Dhont:27208,
author = {Dhont, J. K. G. and Wagner, N. J.},
title = {{S}uperposition rheology},
journal = {Physical review / E},
volume = {63},
number = {2},
issn = {1063-651X},
address = {College Park, Md.},
publisher = {APS},
reportid = {PreJuSER-27208},
pages = {021406},
year = {2001},
note = {Record converted from VDB: 12.11.2012},
abstract = {The interpretation of superposition rheology data is still
a matter of debate due to lack of understanding of
viscoelastic superposition response on a microscopic level.
So far, only phenomenological approaches have been
described, which do not capture the shear induced
microstructural deformation, which is responsible for the
viscoelastic behavior to the superimposed flow.
Experimentally there are indications that there is a
fundamental difference between the viscoelastic response to
an orthogonally and a parallel superimposed shear flow. We
present theoretical predictions, based on microscopic
considerations, for both orthogonal and parallel
viscoelastic response functions for a colloidal system of
attractive particles near their gas-liquid critical point.
These predictions extend to values of the stationary shear
rate where the system is nonlinearly perturbed, and are
based on considerations on the colloidal particle level. The
difference in response to orthogonal and parallel
superimposed shear flow can be understood entirely in terms
of microstructural distortion, where the anisotropy of the
microstructure under shear flow conditions is essential. In
accordance with experimental observations we find pronounced
negative values for response functions in case of parallel
superposition for an intermediate range of frequencies,
provided that microstructure is nonlinearly perturbed by the
stationary shear component. For the critical colloidal
systems considered here, the Kramers-Kronig relations for
the superimposed response Functions are found to be valid.
It is argued, however, that the Kramers-Kronig relations may
be violated for systems where the stationary shear flow
induces a considerable amount of new microstructure.},
keywords = {J (WoSType)},
cin = {IFF-WM},
ddc = {530},
cid = {I:(DE-Juel1)VDB36},
pnm = {Polymere, Membranen und komplexe Flüssigkeiten},
pid = {G:(DE-Juel1)FUEK53},
shelfmark = {Physics, Fluids $\&$ Plasmas / Physics, Mathematical},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000167022300044},
doi = {10.1103/PhysRevE.63.021406},
url = {https://juser.fz-juelich.de/record/27208},
}