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@ARTICLE{Inness:275995,
author = {Inness, A. and Blechschmidt, A.-M. and Bouarar, I. and
Chabrillat, S. and Crepulja, M. and Engelen, R. J. and
Eskes, H. and Flemming, J. and Gaudel, A. and Hendrick, F.
and Huijnen, V. and Jones, L. and Kapsomenakis, J. and
Katragkou, E. and Keppens, A. and Langerock, B. and de
Mazière, M. and Melas, D. and Parrington, M. and Peuch, V.
H. and Razinger, M. and Richter, A. and Schultz, Martin and
Suttie, M. and Thouret, V. and Vrekoussis, M. and Wagner, A.
and Zerefos, C.},
title = {{D}ata assimilation of satellite-retrieved ozone, carbon
monoxide and nitrogen dioxide with {ECMWF}'s
{C}omposition-{IFS}},
journal = {Atmospheric chemistry and physics},
volume = {15},
number = {9},
issn = {1680-7324},
address = {Katlenburg-Lindau},
publisher = {EGU},
reportid = {FZJ-2015-06493},
pages = {5275 - 5303},
year = {2015},
abstract = {Daily global analyses and 5-day forecasts are generated in
the context of the European Monitoring Atmospheric
Composition and Climate (MACC) project using an extended
version of the Integrated Forecasting System (IFS) of the
European Centre for Medium-Range Weather Forecasts (ECMWF).
The IFS now includes modules for chemistry, deposition and
emission of reactive gases, aerosols, and greenhouse gases,
and the 4-dimensional variational data assimilation scheme
makes use of multiple satellite observations of atmospheric
composition in addition to meteorological observations. This
paper describes the data assimilation setup of the new
Composition-IFS (C-IFS) with respect to reactive gases and
validates analysis fields of ozone (O3), carbon monoxide
(CO), and nitrogen dioxide (NO2) for the year 2008 against
independent observations and a control run without data
assimilation. The largest improvement in CO by assimilation
of Measurements of Pollution in the Troposphere (MOPITT) CO
columns is seen in the lower troposphere of the Northern
Hemisphere (NH) extratropics during winter, and during the
South African biomass-burning season. The assimilation of
several O3 total column and stratospheric profile retrievals
greatly improves the total column, stratospheric and upper
tropospheric O3 analysis fields relative to the control run.
The impact on lower tropospheric ozone, which comes from the
residual of the total column and stratospheric profile O3
data, is smaller, but nevertheless there is some improvement
particularly in the NH during winter and spring. The impact
of the assimilation of tropospheric NO2 columns from the
Ozone Monitoring Instrument (OMI) is small because of the
short lifetime of NO2, suggesting that NO2 observations
would be better used to adjust emissions instead of initial
conditions. The results further indicate that the quality of
the tropospheric analyses and of the stratospheric ozone
analysis obtained with the C-IFS system has improved
compared to the previous "coupled" model system of MACC.},
cin = {IEK-8},
ddc = {550},
cid = {I:(DE-Juel1)IEK-8-20101013},
pnm = {243 - Tropospheric trace substances and their
transformation processes (POF3-243) / MACC-III - Monitoring
Atmospheric Composition and Climate -III (633080) / MACC II
- Monitoring Atmospheric Composition and Climate Interim
Implementation (283576)},
pid = {G:(DE-HGF)POF3-243 / G:(EU-Grant)633080 /
G:(EU-Grant)283576},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000355289100019},
doi = {10.5194/acp-15-5275-2015},
url = {https://juser.fz-juelich.de/record/275995},
}