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000276104 1001_ $$0P:(DE-HGF)0$$aRoldin, P.$$b0$$eCorresponding author
000276104 245__ $$aModelling the contribution of biogenic volatile organic compounds to new particle formation in the Jülich plant atmosphere chamber
000276104 260__ $$aKatlenburg-Lindau$$bEGU$$c2015
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000276104 520__ $$aWe used the Aerosol Dynamics gas- and particle-phase chemistry model for laboratory CHAMber studies (ADCHAM) to simulate the contribution of BVOC plant emissions to the observed new particle formation during photooxidation experiments performed in the Jülich Plant-Atmosphere Chamber and to evaluate how well smog chamber experiments can mimic the atmospheric conditions during new particle formation events. ADCHAM couples the detailed gas-phase chemistry from Master Chemical Mechanism with a novel aerosol dynamics and particle phase chemistry module. Our model simulations reveal that the observed particle growth may have either been controlled by the formation rate of semi- and low-volatility organic compounds in the gas phase or by acid catalysed heterogeneous reactions between semi-volatility organic compounds in the particle surface layer (e.g. peroxyhemiacetal dimer formation). The contribution of extremely low-volatility organic gas-phase compounds to the particle formation and growth was suppressed because of their rapid and irreversible wall losses, which decreased their contribution to the nano-CN formation and growth compared to the atmospheric situation. The best agreement between the modelled and measured total particle number concentration (R2 > 0.95) was achieved if the nano-CN was formed by kinetic nucleation involving both sulphuric acid and organic compounds formed from OH oxidation of BVOCs.
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000276104 7001_ $$0P:(DE-HGF)0$$aLiao, L.$$b1
000276104 7001_ $$0P:(DE-HGF)0$$aMogensen, D.$$b2
000276104 7001_ $$0P:(DE-Juel1)7136$$aDal Maso, Miikka$$b3
000276104 7001_ $$0P:(DE-HGF)0$$aRusanen, A.$$b4
000276104 7001_ $$0P:(DE-HGF)0$$aKerminen, V.-M.$$b5
000276104 7001_ $$0P:(DE-Juel1)16346$$aMentel, T. F.$$b6$$ufzj
000276104 7001_ $$0P:(DE-Juel1)129421$$aWildt, J.$$b7$$ufzj
000276104 7001_ $$0P:(DE-Juel1)129345$$aKleist, E.$$b8$$ufzj
000276104 7001_ $$0P:(DE-Juel1)4528$$aKiendler-Scharr, A.$$b9$$ufzj
000276104 7001_ $$0P:(DE-Juel1)5344$$aTillmann, R.$$b10$$ufzj
000276104 7001_ $$0P:(DE-Juel1)144056$$aEhn, M.$$b11
000276104 7001_ $$0P:(DE-HGF)0$$aKulmala, M.$$b12
000276104 7001_ $$0P:(DE-HGF)0$$aBoy, M.$$b13
000276104 773__ $$0PERI:(DE-600)2069847-1$$a10.5194/acp-15-10777-2015$$gVol. 15, no. 18, p. 10777 - 10798$$n18$$p10777 - 10798$$tAtmospheric chemistry and physics$$v15$$x1680-7324$$y2015
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