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@ARTICLE{Roldin:276104,
      author       = {Roldin, P. and Liao, L. and Mogensen, D. and Dal Maso,
                      Miikka and Rusanen, A. and Kerminen, V.-M. and Mentel, T. F.
                      and Wildt, J. and Kleist, E. and Kiendler-Scharr, A. and
                      Tillmann, R. and Ehn, M. and Kulmala, M. and Boy, M.},
      title        = {{M}odelling the contribution of biogenic volatile organic
                      compounds to new particle formation in the {J}ülich plant
                      atmosphere chamber},
      journal      = {Atmospheric chemistry and physics},
      volume       = {15},
      number       = {18},
      issn         = {1680-7324},
      address      = {Katlenburg-Lindau},
      publisher    = {EGU},
      reportid     = {FZJ-2015-06582},
      pages        = {10777 - 10798},
      year         = {2015},
      abstract     = {We used the Aerosol Dynamics gas- and particle-phase
                      chemistry model for laboratory CHAMber studies (ADCHAM) to
                      simulate the contribution of BVOC plant emissions to the
                      observed new particle formation during photooxidation
                      experiments performed in the Jülich Plant-Atmosphere
                      Chamber and to evaluate how well smog chamber experiments
                      can mimic the atmospheric conditions during new particle
                      formation events. ADCHAM couples the detailed gas-phase
                      chemistry from Master Chemical Mechanism with a novel
                      aerosol dynamics and particle phase chemistry module. Our
                      model simulations reveal that the observed particle growth
                      may have either been controlled by the formation rate of
                      semi- and low-volatility organic compounds in the gas phase
                      or by acid catalysed heterogeneous reactions between
                      semi-volatility organic compounds in the particle surface
                      layer (e.g. peroxyhemiacetal dimer formation). The
                      contribution of extremely low-volatility organic gas-phase
                      compounds to the particle formation and growth was
                      suppressed because of their rapid and irreversible wall
                      losses, which decreased their contribution to the nano-CN
                      formation and growth compared to the atmospheric situation.
                      The best agreement between the modelled and measured total
                      particle number concentration (R2 > 0.95) was achieved if
                      the nano-CN was formed by kinetic nucleation involving both
                      sulphuric acid and organic compounds formed from OH
                      oxidation of BVOCs.},
      cin          = {IEK-8 / IBG-2},
      ddc          = {550},
      cid          = {I:(DE-Juel1)IEK-8-20101013 / I:(DE-Juel1)IBG-2-20101118},
      pnm          = {243 - Tropospheric trace substances and their
                      transformation processes (POF3-243)},
      pid          = {G:(DE-HGF)POF3-243},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000362457400028},
      doi          = {10.5194/acp-15-10777-2015},
      url          = {https://juser.fz-juelich.de/record/276104},
}