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| 024 | 7 | _ | |2 doi |a 10.5194/acp-15-10777-2015 |
| 024 | 7 | _ | |2 ISSN |a 1680-7316 |
| 024 | 7 | _ | |2 ISSN |a 1680-7324 |
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| 100 | 1 | _ | |0 P:(DE-HGF)0 |a Roldin, P. |b 0 |e Corresponding author |
| 245 | _ | _ | |a Modelling the contribution of biogenic volatile organic compounds to new particle formation in the Jülich plant atmosphere chamber |
| 260 | _ | _ | |a Katlenburg-Lindau |b EGU |c 2015 |
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| 520 | _ | _ | |a We used the Aerosol Dynamics gas- and particle-phase chemistry model for laboratory CHAMber studies (ADCHAM) to simulate the contribution of BVOC plant emissions to the observed new particle formation during photooxidation experiments performed in the Jülich Plant-Atmosphere Chamber and to evaluate how well smog chamber experiments can mimic the atmospheric conditions during new particle formation events. ADCHAM couples the detailed gas-phase chemistry from Master Chemical Mechanism with a novel aerosol dynamics and particle phase chemistry module. Our model simulations reveal that the observed particle growth may have either been controlled by the formation rate of semi- and low-volatility organic compounds in the gas phase or by acid catalysed heterogeneous reactions between semi-volatility organic compounds in the particle surface layer (e.g. peroxyhemiacetal dimer formation). The contribution of extremely low-volatility organic gas-phase compounds to the particle formation and growth was suppressed because of their rapid and irreversible wall losses, which decreased their contribution to the nano-CN formation and growth compared to the atmospheric situation. The best agreement between the modelled and measured total particle number concentration (R2 > 0.95) was achieved if the nano-CN was formed by kinetic nucleation involving both sulphuric acid and organic compounds formed from OH oxidation of BVOCs. |
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| 700 | 1 | _ | |0 P:(DE-HGF)0 |a Liao, L. |b 1 |
| 700 | 1 | _ | |0 P:(DE-HGF)0 |a Mogensen, D. |b 2 |
| 700 | 1 | _ | |0 P:(DE-Juel1)7136 |a Dal Maso, Miikka |b 3 |
| 700 | 1 | _ | |0 P:(DE-HGF)0 |a Rusanen, A. |b 4 |
| 700 | 1 | _ | |0 P:(DE-HGF)0 |a Kerminen, V.-M. |b 5 |
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| 700 | 1 | _ | |0 P:(DE-Juel1)129345 |a Kleist, E. |b 8 |u fzj |
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| 700 | 1 | _ | |0 P:(DE-Juel1)5344 |a Tillmann, R. |b 10 |u fzj |
| 700 | 1 | _ | |0 P:(DE-Juel1)144056 |a Ehn, M. |b 11 |
| 700 | 1 | _ | |0 P:(DE-HGF)0 |a Kulmala, M. |b 12 |
| 700 | 1 | _ | |0 P:(DE-HGF)0 |a Boy, M. |b 13 |
| 773 | _ | _ | |0 PERI:(DE-600)2069847-1 |a 10.5194/acp-15-10777-2015 |g Vol. 15, no. 18, p. 10777 - 10798 |n 18 |p 10777 - 10798 |t Atmospheric chemistry and physics |v 15 |x 1680-7324 |y 2015 |
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