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@ARTICLE{Chatterji:276107,
author = {Chatterji, Tapan and Kumar, Naveen and Wdowik, Urszula D.},
title = {{A}nomalous temperature-induced volume contraction in
{G}e{T}e},
journal = {Physical review / B},
volume = {91},
number = {5},
issn = {1098-0121},
address = {College Park, Md.},
publisher = {APS},
reportid = {FZJ-2015-06585},
pages = {054110},
year = {2015},
abstract = {The recent surge of interest in phase-change materials
GeTe, Ge2Sb2Te5, and related compounds motivated us to
revisit the structural phase transition in GeTe in more
detail than was done before. The rhombohedral-to-cubic
ferroelectric phase transition in GeTe has been studied
using high-resolution neutron powder diffraction on a
spallation neutron source. We determined the temperature
dependence of the structural parameters in a wide
temperature range extending from 309 to 973 K. The results
of our studies clearly show an anomalous volume contraction
of $0.6\%$ at the phase transition from the
rhombohedral-to-cubic phase. In order to better understand
the phase transition and the associated anomalous volume
decrease in GeTe, we have performed phonon calculations
based on the density functional theory. Results of the
present investigations are also discussed with respect to
the experimental data obtained for single crystals of GeTe.},
cin = {ICS-1 / Neutronenstreuung ; JCNS-1 / JCNS-SNS},
ddc = {530},
cid = {I:(DE-Juel1)ICS-1-20110106 / I:(DE-Juel1)JCNS-1-20110106 /
I:(DE-Juel1)JCNS-SNS-20110128},
pnm = {551 - Functional Macromolecules and Complexes (POF3-551) /
6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)
/ 6215 - Soft Matter, Health and Life Sciences (POF3-621)},
pid = {G:(DE-HGF)POF3-551 / G:(DE-HGF)POF3-6G4 /
G:(DE-HGF)POF3-6215},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000350314100001},
doi = {10.1103/PhysRevB.91.054110},
url = {https://juser.fz-juelich.de/record/276107},
}