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@ARTICLE{Akola:276212,
author = {Akola, J. and Beuneu, B. and Jones, R. O. and Jóvári, P.
and Kaban, I. and Kolář, J. and Voleská, I. and Wágner,
T.},
title = {{S}tructure of amorphous {A}g/{G}e/{S} alloys:
experimentally constrained density functional study},
journal = {Journal of physics / Condensed matter},
volume = {27},
number = {48},
issn = {1361-648X},
address = {Bristol},
publisher = {IOP Publ.},
reportid = {FZJ-2015-06677},
pages = {485304},
year = {2015},
abstract = {Density functional/molecular dynamics simulations have been
performed to determine structural and other properties of
amorphous Ag/Ge/S and Ge/S alloys. In the former, the
calculations have been combined with experimental data
(x-ray and neutron diffraction, extended x-ray absorption
fine structure). Ag/Ge/As alloys have high ionic
conductivity and are among the most promising candidates for
future memristor technology. We find excellent agreement
between the experimental results and large-scale (500 atoms)
simulations in Ag/Ge/S, and we compare and contrast the
structures of Ge/S and Ag/Ge/S. The calculated electronic
structures, vibrational densities of states, ionic
mobilities, and cavity distributions of the amorphous
materials are discussed and compared with data on
crystalline phases where available. The high mobility of Ag
in solid state electrolyte applications is related to the
presence of cavities and can occur via jumps to a
neighbouring vacant site.},
cin = {IAS-1 / PGI-1 / JARA-FIT},
ddc = {530},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106 /
$I:(DE-82)080009_20140620$},
pnm = {142 - Controlling Spin-Based Phenomena (POF3-142) / 143 -
Controlling Configuration-Based Phenomena (POF3-143)},
pid = {G:(DE-HGF)POF3-142 / G:(DE-HGF)POF3-143},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000365346900006},
doi = {10.1088/0953-8984/27/48/485304},
url = {https://juser.fz-juelich.de/record/276212},
}