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@ARTICLE{Rogala:276430,
author = {Rogala, Maciej and Bihlmayer, Gustav and Speier, Wolfgang
and Klusek, Zbigniew and Rodenbücher, Christian and Szot,
K.},
title = {{R}esistive {S}witching of a {Q}uasi-{H}omogeneous
{D}istribution of {F}ilaments {G}enerated at
{H}eat-{T}reated {T}i{O} $_{2}$ (110)-{S}urfaces},
journal = {Advanced functional materials},
volume = {25},
number = {40},
issn = {1616-301X},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2015-06869},
pages = {6382 - 6389},
year = {2015},
abstract = {Resistive switching of thermally treated rutile single
crystals with (110) orientation is studied. A heat treatment
procedure is developed that involves reduction and oxidation
steps and allows to induce low resistance states in
switchable regions at the surface by low-voltage electrical
stimulation with the conducting tip of an atomic force
microscope. This way, it is possible to electrically imprint
quasi-homogeneous switchable regions over several square
micrometers. These regions are identified to consist of
nanofilaments crossing the surface with a density of around
1012 cm−2, much higher in density than observed for single
crystals so far. Experimental evidence is given that these
nanofilaments are not related to inherent structural
imperfections such as dislocations, but may originate from
the linear agglomeration of oxygen vacancies as predicted by
theory. Ab initio calculations and electrical simulations
are performed to analyze the filamentary structures and
their network in the effort to explain the observed
filamentary switching of heat-treated single-crystalline
TiO2.},
cin = {PGI-1 / PGI-7 / UE / IAS-1 / JARA-FIT},
ddc = {620},
cid = {I:(DE-Juel1)PGI-1-20110106 / I:(DE-Juel1)PGI-7-20110106 /
I:(DE-Juel1)UE-20120423 / I:(DE-Juel1)IAS-1-20090406 /
$I:(DE-82)080009_20140620$},
pnm = {142 - Controlling Spin-Based Phenomena (POF3-142)},
pid = {G:(DE-HGF)POF3-142},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000363685900009},
doi = {10.1002/adfm.201500855},
url = {https://juser.fz-juelich.de/record/276430},
}