Hauptseite > Publikationsdatenbank > Melting of Pb Charge Glass and Simultaneous Pb–Cr Charge Transfer in PbCrO $_{3}$ as the Origin of Volume Collapse > print

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024 7 _ |a 10.1021/jacs.5b08216
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245 _ _ |a Melting of Pb Charge Glass and Simultaneous Pb–Cr Charge Transfer in PbCrO $_{3}$ as the Origin of Volume Collapse
260 _ _ |a Washington, DC
|b American Chemical Society
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520 _ _ |a A metal to insulator transition in integer or half integer charge systems can be regarded as crystallization of charges. The insulating state tends to have a glassy nature when randomness or geometrical frustration exists. We report that the charge glass state is realized in a perovskite compound PbCrO3, which has been known for almost 50 years, without any obvious inhomogeneity or triangular arrangement in the charge system. PbCrO3 has a valence state of Pb2+0.5Pb4+0.5Cr3+O3 with Pb2+–Pb4+ correlation length of three lattice-spacings at ambient condition. A pressure induced melting of charge glass and simultaneous Pb–Cr charge transfer causes an insulator to metal transition and ∼10% volume collapse.
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