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000002774 1001_ $$0P:(DE-HGF)0$$aUeba, H.$$b0
000002774 245__ $$aAdsorbate hopping via vibrational-mode coupling induced by femtosecond laser pulses
000002774 260__ $$aCollege Park, Md.$$bAPS$$c2008
000002774 300__ $$a113408
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000002774 500__ $$aWe thank M. Bonn for critical reading of the manuscript and valuable comments and U. Hofer for useful discussions. The present work was supported by the Grant-in-Aid for Scientific Research B (No. 18340085) from the Japan Society for the Promotion of Science.
000002774 520__ $$aWe study the heat transfer from femtosecond laser-heated hot electrons in a metal to adsorbates in the presence of vibrational-mode coupling. The theory is successfully applied to the experimental result of atomic oxygen hopping on a vicinal Pt(111) surface. The effective friction coupling between hot electrons and the vibrational mode relevant to the hopping motion depends on the transient temperature of the partner mode excited by hot electrons. The calculated two-pulse correlation and fluence dependence of the hopping probability reproduce the experimental results, which were previously analyzed using the hot-electron temperature (Te)-dependent friction eta(a)(Te) in a conventional heat transfer equation. A possible elementary process behind such a hypothetic modeling using eta(a)(Te) is discussed in terms of an indirect heating of the vibrational mode for hopping at the surface.
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000002774 7001_ $$0P:(DE-HGF)0$$aHayashi, M.$$b1
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000002774 7001_ $$0P:(DE-Juel1)130885$$aPersson, B. N. J.$$b3$$uFZJ
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