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@ARTICLE{Rosati:278668,
author = {Rosati, B. and Herrmann, E. and Bucci, S. and Fierli, F.
and Cairo, F. and Gysel, M. and Tillmann, R. and Größ, J.
and Gobbi, G. P. and Di Liberto, L. and Di Donfrancesco, G.
and Wiedensohler, A. and Weingartner, E. and Virtanen, A.
and Mentel, T. F. and Baltensperger, U.},
title = {{C}omparison of vertical aerosol extinction coefficients
from in-situ and {LIDAR} measurements},
journal = {Atmospheric chemistry and physics / Discussions},
volume = {15},
number = {13},
issn = {1680-7375},
address = {Katlenburg-Lindau},
publisher = {EGU},
reportid = {FZJ-2015-06993},
pages = {18609 - 18651},
year = {2015},
abstract = {Vertical profiles of aerosol optical properties were
explored in a case study near the San Pietro Capofiume (SPC)
ground station during the PEGASOS Po Valley campaign in the
summer of 2012. A Zeppelin NT airship was employed to
investigate the effect of the dynamics of the planetary
boundary layer at altitudes between ~ 50–800 m above
ground. Determined properties included the aerosol size
distribution, the hygroscopic growth factor, the effective
index of refraction and the light absorption coefficient.
The first three parameters were used to retrieve the light
scattering coefficient. Simultaneously, direct measurements
of both the scattering and absorption coefficient were
carried out at the SPC ground station. Additionally, a LIDAR
system provided aerosol extinction coefficients for a
vertically resolved comparison between in-situ and remote
sensing results. First, the airborne results at low
altitudes were validated with the ground measurements.
Agreement within approximately ±25 and $±20\%$ was found
for the dry scattering and absorption coefficient,
respectively. The single scattering albedo, ranged between
0.83 to 0.95, indicating the importance of the absorbing
particles in the Po Valley region. A clear layering of the
atmosphere was observed during the beginning of the flight
(until ~ 10 local time) before the mixed layer (ML) was
fully developed. Highest extinction coefficients were found
at low altitudes, in the new ML, while values in the
residual layer, which could be probed at the beginning of
the flight at elevated altitudes, were lower. At the end of
the flight (after ~ 12 local time) the ML was fully
developed, resulting in constant extinction coefficients at
all altitudes measured on the Zeppelin NT. LIDAR results
captured these dynamic features well and good agreement was
found for the extinction coefficients compared to the
in-situ results, using fixed LIDAR ratios (LR) between 30
and 70 sr for the altitudes probed with the Zeppelin. These
LR are consistent with values for continental aerosol
particles that can be expected in this region.},
cin = {IEK-8},
ddc = {550},
cid = {I:(DE-Juel1)IEK-8-20101013},
pnm = {243 - Tropospheric trace substances and their
transformation processes (POF3-243)},
pid = {G:(DE-HGF)POF3-243},
typ = {PUB:(DE-HGF)16},
doi = {10.5194/acpd-15-18609-2015},
url = {https://juser.fz-juelich.de/record/278668},
}