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@ARTICLE{Niedrig:278804,
author = {Niedrig, Christian and Wagner, Stefan F. and Menesklou,
Wolfgang and Baumann, Stefan and Ivers-Tiffée, Ellen},
title = {{O}xygen equilibration kinetics of mixed-conducting
perovskites {BSCF}, {LSCF}, and {PSCF} at 900°{C}
determined by electrical conductivity relaxation},
journal = {Solid state ionics},
volume = {283},
issn = {0167-2738},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2015-07037},
pages = {30-37},
year = {2015},
abstract = {For an application of mixed ionic-electronic conducting
(MIEC) perovskite oxides, e.g., as solid oxide fuel cell
(SOFC) cathodes, as high-temperature gas sensors or as
oxygen-transport membrane (OTM) materials, the kinetics of
oxygen transport is of fundamental importance.A common setup
for the determination of the chemical diffusion coefficient
Dδ and the surface exchange coefficient kδ is the
electrical conductivity relaxation (ECR) method where the
conductivity response of an MIEC sample is measured after
the ambient oxygen partial pressure pO2 has been abruptly
changed using different gas mixtures. In the present study,
however, a closed tubular zirconia “oxygen pump” setup
was used which facilitates precise pO2 control in a closed
sample space with a high resolution at temperatures above
700 °C in atmospheres ranging from pure oxygen continuously
down to pO2 = 10− 18 bar. Reasonably fast pO2 changes
enable an application of the ECR technique on MIEC oxides
down to lower partial pressures not easily accessible with
gas mixtures.The oxygen transport parameters of dense
ceramic bulk samples of Ba0.5Sr0.5Co0.8Fe0.2O3 -δ (BSCF),
La0.58Sr0.4Co0.2Fe0.8O3 -δ (LSCF), and
Pr0.58Sr0.4Co0.2Fe0.8O3 -δ (PSCF) have been studied as a
function of temperature (800 and 900 °C) in the range
between 10− 6 ≤ pO2/bar ≤ 0.21. The Dδ and kδ values
obtained for LSCF at 800 °C are in good agreement with
values from literature, proving the usability of the setup
for ECR measurements. For BSCF, LSCF, and PSCF, Dδ and kδ
values could be determined for the first time at 900 °C as
a function of pO2.},
cin = {IEK-1},
ddc = {530},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {113 - Methods and Concepts for Material Development
(POF3-113)},
pid = {G:(DE-HGF)POF3-113},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000367113100005},
doi = {10.1016/j.ssi.2015.11.004},
url = {https://juser.fz-juelich.de/record/278804},
}