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@ARTICLE{Navarro:280913,
author = {Navarro, P. and Bocquet, F. C. and Deperasińska, I. and
Pirug, G. and Tautz, F. S. and Orrit, M.},
title = {{E}lectron {E}nergy {L}oss of {T}errylene {D}eposited on
{A}u(111): {V}ibrational and {E}lectronic {S}pectroscopy},
journal = {The journal of physical chemistry / C},
volume = {119},
number = {1},
issn = {1932-7455},
address = {Washington, DC},
publisher = {Soc.},
reportid = {FZJ-2016-00624},
pages = {277 - 283},
year = {2015},
abstract = {We have investigated the vibrational and electronic
properties of terrylene by high-resolution electron
energy-loss spectroscopy (HREELS), Fourier-transform
infrared spectroscopy, and low-temperature single-molecule
fluorescence spectroscopy. Terrylene thin films were
sublimated in an ultrahigh vacuum on the Au(111) surface in
order to record the HREEL spectra. Polycrystalline
p-dichlorobenzene was used as a matrix to isolate a single
terrylene molecule at 1.5 K and record its fluorescence
spectrum. The infrared spectrum, the vibrational components
from the fluorescence spectrum, and density functional
theory calculations were used for the assignment and
identification of the active modes found in HREELS. Finally,
we report a loss signal around 17 000 cm–1 (2.1 eV) for
the first singlet electronic excited state in agreement with
optical spectroscopy. The HREEL spectra show both IR- and
Raman-active vibration modes because of specific surface
selection rules. Energy-loss spectroscopy could be used as a
complementary technique to explore some other degrees of
freedom that are not accessible by optical means.},
cin = {PGI-3 / JARA-FIT},
ddc = {540},
cid = {I:(DE-Juel1)PGI-3-20110106 / $I:(DE-82)080009_20140620$},
pnm = {141 - Controlling Electron Charge-Based Phenomena
(POF3-141)},
pid = {G:(DE-HGF)POF3-141},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000347744700031},
doi = {10.1021/jp5086262},
url = {https://juser.fz-juelich.de/record/280913},
}