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001     281044
005     20210129221611.0
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100 1 _ |0 P:(DE-HGF)0
|a Huttmann, Felix
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245 _ _ |a Tuning the van der Waals Interaction of Graphene with Molecules via Doping
260 _ _ |a College Park, Md.
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520 _ _ |a We use scanning tunneling microscopy to visualize and thermal desorption spectroscopy to quantitatively measure that the binding of naphthalene molecules to graphene, a case of pure van der Waals interaction, strengthens with n and weakens with p doping of graphene. Density-functional theory calculations that include the van der Waals interaction in a seamless, ab initio way accurately reproduce the observed trend in binding energies. Based on a model calculation, we propose that the van der Waals interaction is modified by changing the spatial extent of graphene’s π orbitals via doping.
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