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000281958 1001_ $$0P:(DE-HGF)0$$aSteinbrecher, M.$$b0$$eCorresponding author
000281958 245__ $$aAbsence of a spin-signature from a single Ho adatom as probed by spin-sensitive tunneling
000281958 260__ $$aLondon$$bNature Publishing Group$$c2016
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000281958 520__ $$aWhether rare-earth materials can be used as single-atom magnetic memory is an ongoing debate in recent literature. Here we show, by inelastic and spin-resolved scanning tunnelling-based methods, that we observe a strong magnetic signal and excitation from Fe atoms adsorbed on Pt(111), but see no signatures of magnetic excitation or spin-based telegraph noise for Ho atoms. Moreover, we observe that the indirect exchange field produced by a single Ho atom is negligible, as sensed by nearby Fe atoms. We demonstrate, using ab initio methods, that this stems from a comparatively weak coupling of the Ho 4f electrons with both tunnelling electrons and substrate-derived itinerant electrons, making both magnetic coupling and detection very difficult when compared to 3d elements. We discuss these results in the context of ongoing disputes and clarify important controversies.
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000281958 7001_ $$0P:(DE-HGF)0$$aSonntag, A.$$b1
000281958 7001_ $$0P:(DE-Juel1)145395$$ados Santos Dias, Manuel$$b2
000281958 7001_ $$0P:(DE-Juel1)145203$$aBouhassoune, M.$$b3
000281958 7001_ $$0P:(DE-Juel1)130805$$aLounis, S.$$b4$$eCorresponding author
000281958 7001_ $$0P:(DE-HGF)0$$aWiebe, J.$$b5
000281958 7001_ $$0P:(DE-HGF)0$$aWiesendanger, R.$$b6
000281958 7001_ $$0P:(DE-HGF)0$$aKhajetoorians, A. A.$$b7
000281958 773__ $$0PERI:(DE-600)2553671-0$$a10.1038/ncomms10454$$gVol. 7, p. 10454 -$$p10454$$tNature Communications$$v7$$x2041-1723$$y2016
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