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@ARTICLE{Steinbrecher:281958,
author = {Steinbrecher, M. and Sonntag, A. and dos Santos Dias,
Manuel and Bouhassoune, M. and Lounis, S. and Wiebe, J. and
Wiesendanger, R. and Khajetoorians, A. A.},
title = {{A}bsence of a spin-signature from a single {H}o adatom as
probed by spin-sensitive tunneling},
journal = {Nature Communications},
volume = {7},
issn = {2041-1723},
address = {London},
publisher = {Nature Publishing Group},
reportid = {FZJ-2016-01602},
pages = {10454},
year = {2016},
abstract = {Whether rare-earth materials can be used as single-atom
magnetic memory is an ongoing debate in recent literature.
Here we show, by inelastic and spin-resolved scanning
tunnelling-based methods, that we observe a strong magnetic
signal and excitation from Fe atoms adsorbed on Pt(111), but
see no signatures of magnetic excitation or spin-based
telegraph noise for Ho atoms. Moreover, we observe that the
indirect exchange field produced by a single Ho atom is
negligible, as sensed by nearby Fe atoms. We demonstrate,
using ab initio methods, that this stems from a
comparatively weak coupling of the Ho 4f electrons with both
tunnelling electrons and substrate-derived itinerant
electrons, making both magnetic coupling and detection very
difficult when compared to 3d elements. We discuss these
results in the context of ongoing disputes and clarify
important controversies.},
cin = {IAS-1 / PGI-1 / JARA-FIT},
ddc = {500},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106 /
$I:(DE-82)080009_20140620$},
pnm = {142 - Controlling Spin-Based Phenomena (POF3-142)},
pid = {G:(DE-HGF)POF3-142},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000371135900001},
doi = {10.1038/ncomms10454},
url = {https://juser.fz-juelich.de/record/281958},
}