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001     281958
005     20210129222124.0
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100 1 _ |a Steinbrecher, M.
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245 _ _ |a Absence of a spin-signature from a single Ho adatom as probed by spin-sensitive tunneling
260 _ _ |a London
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520 _ _ |a Whether rare-earth materials can be used as single-atom magnetic memory is an ongoing debate in recent literature. Here we show, by inelastic and spin-resolved scanning tunnelling-based methods, that we observe a strong magnetic signal and excitation from Fe atoms adsorbed on Pt(111), but see no signatures of magnetic excitation or spin-based telegraph noise for Ho atoms. Moreover, we observe that the indirect exchange field produced by a single Ho atom is negligible, as sensed by nearby Fe atoms. We demonstrate, using ab initio methods, that this stems from a comparatively weak coupling of the Ho 4f electrons with both tunnelling electrons and substrate-derived itinerant electrons, making both magnetic coupling and detection very difficult when compared to 3d elements. We discuss these results in the context of ongoing disputes and clarify important controversies.
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700 1 _ |a Sonntag, A.
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700 1 _ |a dos Santos Dias, Manuel
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700 1 _ |a Bouhassoune, M.
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700 1 _ |a Lounis, S.
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700 1 _ |a Wiebe, J.
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700 1 _ |a Wiesendanger, R.
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700 1 _ |a Khajetoorians, A. A.
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