000283530 001__ 283530
000283530 005__ 20240712084512.0
000283530 0247_ $$2doi$$a10.1002/pssa.201533025
000283530 0247_ $$2ISSN$$a0031-8965
000283530 0247_ $$2ISSN$$a1521-396X
000283530 0247_ $$2ISSN$$a1862-6300
000283530 0247_ $$2ISSN$$a1862-6319
000283530 0247_ $$2WOS$$aWOS:000385222900013
000283530 037__ $$aFZJ-2016-01849
000283530 041__ $$aEnglish
000283530 082__ $$a530
000283530 1001_ $$0P:(DE-Juel1)142337$$aBecker, Jan Philipp$$b0$$eCorresponding author$$ufzj
000283530 245__ $$aModeling and practical realization of thin film silicon-based integrated solar water splitting devices
000283530 260__ $$aWeinheim$$bWiley-VCH$$c2016
000283530 3367_ $$2DRIVER$$aarticle
000283530 3367_ $$2DataCite$$aOutput Types/Journal article
000283530 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1469435614_12103
000283530 3367_ $$2BibTeX$$aARTICLE
000283530 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000283530 3367_ $$00$$2EndNote$$aJournal Article
000283530 520__ $$aAn integrated solar water splitting device based on thin film silicon multijunction photocathodes is presented. A graphical representation of the photovoltaic current–voltage data is introduced which allows for an estimation of the maximum achievable solar-to-hydrogen efficiency of the integrated device. Furthermore, a simple yet very useful series circuit model is used to predict the photoelectrochemical performance of the integrated device in a more elaborate way when the j–V characteristics of the individual components are known. Within the model, the j–V characteristics of each component can be either modeled with parameters from the literature or measured. The photocathode, the electrolyte concentration, and the hydrogen and oxygen evolving catalysts were varied exemplarily and the impact of each component on the integrated device performance was evaluated. A maximum solar-to-hydrogen efficiency of 9.5% was found using a triple junction solar cell functionalized with a Pt catalyst for the hydrogen evolution and a RuO2 catalyst for the oxygen evolution reaction in a 1 M KOH electrolyte. This result was confirmed experimentally and is compared to efficiencies reported in the literature.
000283530 536__ $$0G:(DE-HGF)POF3-126$$a126 - Solar Fuels (POF3-126)$$cPOF3-126$$fPOF III$$x0
000283530 536__ $$0G:(DE-HGF)POF3-121$$a121 - Solar cells of the next generation (POF3-121)$$cPOF3-121$$fPOF III$$x1
000283530 536__ $$0G:(DE-Juel1)HITEC-20170406$$aHITEC - Helmholtz Interdisciplinary Doctoral Training in Energy and Climate Research (HITEC) (HITEC-20170406)$$cHITEC-20170406$$x2
000283530 588__ $$aDataset connected to CrossRef
000283530 7001_ $$0P:(DE-Juel1)156469$$aUrbain, Félix$$b1$$ufzj
000283530 7001_ $$0P:(DE-Juel1)130297$$aSmirnov, Vladimir$$b2$$ufzj
000283530 7001_ $$0P:(DE-Juel1)143905$$aRau, Uwe$$b3$$ufzj
000283530 7001_ $$0P:(DE-HGF)0$$aZiegler, Jürgen$$b4
000283530 7001_ $$0P:(DE-HGF)0$$aKaiser, Bernhard$$b5
000283530 7001_ $$0P:(DE-HGF)0$$aJaegermann, Wolfram$$b6
000283530 7001_ $$0P:(DE-Juel1)130238$$aFinger, Friedhelm$$b7$$ufzj
000283530 773__ $$0PERI:(DE-600)1481091-8$$a10.1002/pssa.201533025$$gp. n/a - n/a$$n7$$p1738 - 1746$$tPhysica status solidi / A$$v213$$x0031-8965$$y2016
000283530 8564_ $$uhttps://juser.fz-juelich.de/record/283530/files/Becker_et_al-2016-physica_status_solidi_%28a%29.pdf$$yRestricted
000283530 8564_ $$uhttps://juser.fz-juelich.de/record/283530/files/Becker_et_al-2016-physica_status_solidi_%28a%29.gif?subformat=icon$$xicon$$yRestricted
000283530 8564_ $$uhttps://juser.fz-juelich.de/record/283530/files/Becker_et_al-2016-physica_status_solidi_%28a%29.jpg?subformat=icon-1440$$xicon-1440$$yRestricted
000283530 8564_ $$uhttps://juser.fz-juelich.de/record/283530/files/Becker_et_al-2016-physica_status_solidi_%28a%29.jpg?subformat=icon-180$$xicon-180$$yRestricted
000283530 8564_ $$uhttps://juser.fz-juelich.de/record/283530/files/Becker_et_al-2016-physica_status_solidi_%28a%29.jpg?subformat=icon-640$$xicon-640$$yRestricted
000283530 8564_ $$uhttps://juser.fz-juelich.de/record/283530/files/Becker_et_al-2016-physica_status_solidi_%28a%29.pdf?subformat=pdfa$$xpdfa$$yRestricted
000283530 909CO $$ooai:juser.fz-juelich.de:283530$$pVDB
000283530 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)142337$$aForschungszentrum Jülich GmbH$$b0$$kFZJ
000283530 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)156469$$aForschungszentrum Jülich GmbH$$b1$$kFZJ
000283530 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130297$$aForschungszentrum Jülich GmbH$$b2$$kFZJ
000283530 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)143905$$aForschungszentrum Jülich GmbH$$b3$$kFZJ
000283530 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130238$$aForschungszentrum Jülich GmbH$$b7$$kFZJ
000283530 9131_ $$0G:(DE-HGF)POF3-126$$1G:(DE-HGF)POF3-120$$2G:(DE-HGF)POF3-100$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$aDE-HGF$$bEnergie$$lErneuerbare Energien$$vSolar Fuels$$x0
000283530 9131_ $$0G:(DE-HGF)POF3-121$$1G:(DE-HGF)POF3-120$$2G:(DE-HGF)POF3-100$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$aDE-HGF$$bEnergie$$lErneuerbare Energien$$vSolar cells of the next generation$$x1
000283530 9141_ $$y2016
000283530 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS
000283530 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bPHYS STATUS SOLIDI A : 2014
000283530 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection
000283530 915__ $$0StatID:(DE-HGF)0110$$2StatID$$aWoS$$bScience Citation Index
000283530 915__ $$0StatID:(DE-HGF)0111$$2StatID$$aWoS$$bScience Citation Index Expanded
000283530 915__ $$0StatID:(DE-HGF)9900$$2StatID$$aIF < 5
000283530 915__ $$0StatID:(DE-HGF)0550$$2StatID$$aNo Authors Fulltext
000283530 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences
000283530 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline
000283530 915__ $$0StatID:(DE-HGF)0420$$2StatID$$aNationallizenz
000283530 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bThomson Reuters Master Journal List
000283530 920__ $$lyes
000283530 9201_ $$0I:(DE-Juel1)IEK-5-20101013$$kIEK-5$$lPhotovoltaik$$x0
000283530 980__ $$ajournal
000283530 980__ $$aVDB
000283530 980__ $$aUNRESTRICTED
000283530 980__ $$aI:(DE-Juel1)IEK-5-20101013
000283530 981__ $$aI:(DE-Juel1)IMD-3-20101013