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| Hauptseite > Workflowsammlungen > Öffentliche Einträge > Radio frequency magnetron sputtering of Li7La3Zr2O12 thin films for solid-state batteries > print |
| Hauptseite > Workflowsammlungen > Öffentliche Einträge > Radio frequency magnetron sputtering of Li7La3Zr2O12 thin films for solid-state batteries > print |
| 001 | 283555 | ||
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| 100 | 1 | _ | |a Lobe, Sandra |0 P:(DE-Juel1)161444 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Radio frequency magnetron sputtering of Li7La3Zr2O12 thin films for solid-state batteries |
| 260 | _ | _ | |a New York, NY [u.a.] |c 2016 |b Elsevier |
| 336 | 7 | _ | |a Journal Article |b journal |m journal |0 PUB:(DE-HGF)16 |s 1458052101_16395 |2 PUB:(DE-HGF) |
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| 520 | _ | _ | |a Thin film batteries based on solid electrolytes having a garnet-structure like Li7La3Zr2O12 (LLZ) are considered as one option for safer batteries with increased power density. In this work we show the deposition of Ta- and Al-substituted LLZ thin films on stainless steel substrates by r.f. magnetron sputtering. The thin films were characterized by XRD, SEM and time-of-flight-secondary ion mass spectrometry (ToF-SIMS) to determine crystal structure, morphology and element distribution. The substrate temperature was identified to be one important parameter for the formation of cubic garnet-structured LLZ thin films. LLZ formation starts at around 650 °C. Single phase cubic thin films were obtained at substrate temperatures of 700 °C and higher. At these temperatures an interlayer is formed. Combination of SEM, ToF-SIMS and XRD indicated that this layer consists of γ-LiAlO2. The combined total ionic conductivity of the γ-LiAlO2 interlayer and the LLZ thin film (perpendicular to the plane) was determined to be 2.0 × 10−9 S cm−1 for the sample deposited at 700 °C. In-plane measurements showed a room temperature conductivity of 1.2 × 10−4 S cm−1 with an activation energy of 0.47 eV for the LLZ thin film. |
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| 773 | _ | _ | |a 10.1016/j.jpowsour.2015.12.054 |g Vol. 307, p. 684 - 689 |0 PERI:(DE-600)1491915-1 |p 684 - 689 |t Journal of power sources |v 307 |y 2016 |x 0378-7753 |
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