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@ARTICLE{Tietz:283682,
author = {Tietz, F. and Arul Raj, I. and Ma, Q. and Baumann, S. and
Mahmoud, A. and Hermann, Raphael},
title = {{M}aterial properties of perovskites in the quasi-ternary
system
{L}a{F}e{O}$_{3}$–{L}a{C}o{O}$_{3}$–{L}a{N}i{O}$_{3}},
journal = {Journal of solid state chemistry},
volume = {237},
issn = {0022-4596},
address = {Orlando, Fla.},
publisher = {Academic Press},
reportid = {FZJ-2016-01979},
pages = {183 - 191},
year = {2016},
abstract = {An overview is presented on the variation of electrical
conductivity, oxygen permeation, and thermal expansion
coefficient as a function of the composition of perovskites
in the quasi-ternary system LaFeO3–LaCoO3–LaNiO3.
Powders of thirteen nominal perovskite compositions were
synthesized under identical conditions by the Pechini
method. The powder X-ray diffraction data of two series,
namely La(Ni0.5Fe0.5)1−xCoxO3 and LaNi0.5-xFexCo0.5O3, are
presented after the powders had been sintered at 1100 °C
for 6 h in air. The measurements revealed a rhombohedral
structure for all compositions except LaNi0.5Fe0.5O3 for
which $60\%$ rhombohedral and $40\%$ orthorhombic phase was
found. The maximum DC electrical conductivity value of the
perovskites at 800 °C was 1229 S cm−1 for the composition
LaCoO3 and the minimum was 91 S cm−1 for the composition
LaCo0.5Fe0.5O3. The oxygen permeation of samples with
promising conductivities at 800 °C was one order of
magnitude lower than that of La0.6Sr0.4Co0.8Fe0.2O3 (LSCF).
The highest value of 0.017 ml cm−2 min−1 at 950 °C was
obtained with LaNi0.5Co0.5O3. The coefficients of thermal
expansion varied in the range of 13.2×10−6 K−1 and
21.9×10−6 K−1 for LaNi0.5Fe0.5O3 and LaCoO3,
respectively. 57Fe Mössbauer spectroscopy was used as probe
for the oxidation states, local environment and magnetic
properties of iron ions as a function of chemical
composition. The substitution had a great influence on the
chemical properties of the materials.},
cin = {JCNS-2 / PGI-4 / JARA-FIT / IEK-1},
ddc = {540},
cid = {I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)PGI-4-20110106 /
$I:(DE-82)080009_20140620$ / I:(DE-Juel1)IEK-1-20101013},
pnm = {144 - Controlling Collective States (POF3-144) / 524 -
Controlling Collective States (POF3-524) / 6212 - Quantum
Condensed Matter: Magnetism, Superconductivity (POF3-621) /
6213 - Materials and Processes for Energy and Transport
Technologies (POF3-621) / 6G4 - Jülich Centre for Neutron
Research (JCNS) (POF3-623)},
pid = {G:(DE-HGF)POF3-144 / G:(DE-HGF)POF3-524 /
G:(DE-HGF)POF3-6212 / G:(DE-HGF)POF3-6213 /
G:(DE-HGF)POF3-6G4},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000373661100026},
doi = {10.1016/j.jssc.2016.01.024},
url = {https://juser.fz-juelich.de/record/283682},
}